2021
DOI: 10.1525/elementa.2021.00015
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Evolution of formaldehyde (HCHO) in a plume originating from a petrochemical industry and its volatile organic compounds (VOCs) emission rate estimation

Abstract: Large industrial facilities, such as petrochemical complexes, have decisive effects on regional air quality: directly due to their own hazardous volatile organic compounds (VOCs) emissions and indirectly due to their contribution to secondary air pollution. In South Korea, pronounced ozone and particulate matter issues have been reported in industrial areas. In this study, we develop a new top-down VOC emission rate estimation method using in situ airborne formaldehyde (HCHO) observations in the downwind plume… Show more

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Cited by 10 publications
(3 citation statements)
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“…These results were corroborated by a top-down estimate based on CH 2 O column densities remotely sensed by GeoTASO ( Kwon et al, 2021 ) that exceeded the bottom-up inventory by a factor of 4.0 ± 2.3. The third top-down estimate by Cho et al (n.d.) used a box model to evaluate the build-up in CH 2 O between downwind plumes of the Daesan facility sampled by the DC-8 and Hanseo King Air separated by approximately 4.5 h. This resulted in a value that exceeded the bottom-up inventory by a factor of 2.5 ± 0.4.…”
Section: Korus-aq Findings Related To Controlling Factors For Air Qua...mentioning
confidence: 98%
“…These results were corroborated by a top-down estimate based on CH 2 O column densities remotely sensed by GeoTASO ( Kwon et al, 2021 ) that exceeded the bottom-up inventory by a factor of 4.0 ± 2.3. The third top-down estimate by Cho et al (n.d.) used a box model to evaluate the build-up in CH 2 O between downwind plumes of the Daesan facility sampled by the DC-8 and Hanseo King Air separated by approximately 4.5 h. This resulted in a value that exceeded the bottom-up inventory by a factor of 2.5 ± 0.4.…”
Section: Korus-aq Findings Related To Controlling Factors For Air Qua...mentioning
confidence: 98%
“…Laboratories usually perform monitoring by sampling and analysis using liquid chromatography. The number of sensors for measuring HCHO is limited [37], and there are no cheap, accurate, and sensitive HCHO sensors which can determine low concentrations of formaldehyde with sufficient accuracy.…”
Section: Limitations Of Different Air Pollution Monitoring Technologi...mentioning
confidence: 99%
“…Methane (CH4), ethane (C2H6), and propane (C3H8) are the main compounds of natural gas which may often remain dissolved in crude oil samples after separation and consequentially are released alongside vented VOCs. In addition to degrading air quality, these hydrocarbons can be especially damaging to the environment as they undergo photochemical reactions with nitrogen oxides (NOx) and other compounds in the troposphere, resulting in the production of thermal trapping GHGs which can influence weather patterns and severe weather events, and contribute to climate change through global warming (Cho et al, 2021).…”
Section: Introductionmentioning
confidence: 99%