2024
DOI: 10.1021/acsami.3c17730
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Exceptional Thermoelectric Performance of Cu2(Zn,Fe,Cd)SnS4 Thin Films

Yu Liu,
Paul D. McNaughter,
Xiaodong Liu
et al.

Abstract: High-quality Cu 2 (Zn,Fe,Cd)SnS 4 (CZFCTS) thin films based on the parent CZTS were prepared by aerosol-assisted chemical vapor deposition (AACVD). Substitution of Zn by Fe and Cd significantly improved the electrical transport properties, and monophasic CZFCTS thin films exhibited a maximum power factor (PF) of ∼0.22 μW cm −1 K −2 at 575 K. The quality and performance of the CZFCTS thin films were further improved by postdeposition annealing. CZFCTS thin films annealed for 24 h showed a significantly enhanced… Show more

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