Quantum information processing holds great promise for pushing beyond the current frontiers in computing. Specifically, quantum computation promises to accelerate the solving of certain problems, and there are many opportunities for innovation based on applications in chemistry, engineering, and finance. To harness the full potential of quantum computing, however, we must not only place emphasis on manufacturing better qubits, advancing our algorithms, and developing quantum software. To scale devices to the fault tolerant regime, we must refine device-level quantum control.On May 17-18, 2021, the Chicago Quantum Exchange (CQE) partnered with IBM Quantum and Super.tech to host the Pulselevel Quantum Control Workshop. At the workshop, representatives from academia, national labs, and industry addressed the importance of fine-tuning quantum processing at the physical layer. The purpose of this report is to summarize the topics of this meeting for the quantum community at large.