Isotope shifts, spins, hyperfine structures and masses have been measured for the series of the alkali isotopes including the nuclei far from stability. The method of laser spectroscopy and its combinations with rf excitation are described. Some results are discussed, namely the first observation of the red doublet D~-D2 of francium, and the study of shell effects and changes of shape with mass and 6 (r 2 ) measurements for Rb and Na isotopes.
IntroductionThe aim of the experiments which are described here was to study the groundstate properties of the nucleus as a function of the neutron number. Up to now, these experiments were conducted on the series of alkali isotopes since they are particularly suitable for laser spectroscopy as well as for mass measurements. As shown in fig. 1, we have studied the shell effects (N = 20, 28, 50, 82, 126), the odd-even staggerings, the shape isomerisms and the occurrence of deformations. We have tried to measure as many properties as possible concerning the same nuclei in order to obtain cross information.On one hand, we measured the spin I, the magnetic moment ~, the spectroscopic electric quadrupole moment Qs, and the variation of the mean square charge radius 6 (r 2 ) by on-line laser spectroscopy eventually combined with a radio frequency excitation, and on the other, we measured the masses M by on-line mass spectrometry.The nuclei far from stability have been produced using three different kinds of nuclear reactions: the spallation, the fission and the fragmentation by high-energy protons (see fig. 1). These experiments were performed either at ISOLDE, which is a mass separator on line with the S.C. (600 MeV protons) at CERN, or directly on line with the P.S.