The AMPTE (Active Magnetospheric Particle Tracer Explorers) mission provided in situ measurements of collisionless momentum and energy exchange between an artificial, photo-ionized barium plasma cloud and the streaming, magnetized hydrogen plasma of the solar wind [1][2][3] . One of its most significant findings was the unanticipated displacement of the barium ion 'comet head' (and an oppositely directed deflection of the streaming hydrogen ions) transverse to both the solar wind flow and the interplanetary magnetic field, defying the conventional expectation that the barium ions would simply move downwind , a collisionless momentum exchange mechanism believed to occur in various astrophysical and space-plasma environments 10,11 and to participate in cosmic magnetized collisionless shock formation [12][13][14] . Here we present the detection of Larmor coupling in a reproducible laboratory experiment that combines an explosive laser-produced plasma cloud with preformed, magnetized ambient plasma in a parameter regime relevant to the AMPTE barium releases. In our experiment, time-resolved Doppler spectroscopy reveals ambient ion acceleration transverse to both the laser-produced plasma flow and the background magnetic field. Utilizing a detailed numerical simulation, we demonstrate that the ambient ion velocity distribution corresponding to the measured Doppler-shifted spectrum is qualitatively and quantitatively consistent with Larmor coupling.The AMPTE barium release experiments aimed to better understand a ubiquitous category of astrophysical and space phenomena characterized by the rapid expansion or relative motion of a dense 'debris' plasma cloud through relatively tenuous, magnetized, ambient plasma. Examples include the expansion of stellar material through the surrounding interstellar medium in supernova remnants 10 , the formation of cometary plasma tails due to the solar wind 15 , the interaction of interplanetary coronal mass ejections with the Earth's magnetosphere 16 , and man-made ionospheric explosions 17 . In these rarified environments, the Coulomb collisional mean free paths exceed the observed interaction length scales by many orders of magnitude, signifying that the debris plasma exchanges momentum and energy with the ambient plasma via collisionless, collective, electromagnetic effects. In addition, the relative motion of the debris cloud produces electric polarization fields between the magnetically confined electrons and the relatively freestreaming ions, resulting in E × B drift electron currents that expel the magnetic field within the cloud volume (the diamagnetic cavity) and enhance it at the cloud edge (the magnetic compression) 18 . The general evolution in the reference frame of the magnetized ambient plasma is thus a deceleration of the debris cloud as it couples to the ambient plasma via collisionless processes and deforms the magnetic field.We here consider explosive astrophysical and space environments characterized by a perpendicular-to-B debris plasma flow speed V d that exceed...