Based on the inorganic modification of raw soil materials by using cement, fly ash, lime and other admixtures, the influence of modified jute fiber content on the strength of raw-soil-based wall materials was studied. The effects of the gradient distribution of inorganic admixtures on the mechanical properties and thermal conductivity of raw-soil-based wall materials were studied and compared by designing the gradient distribution and homogenous distribution of admixtures in raw soil materials. The results show that when the mass ratio of raw soil, sand, cement, fly ash and lime is 30:10:5:3:2, the compressive strength and flexural strength of the modified raw soil specimen at 28 d are 6.4 MPa and 2.9 MPa, respectively; on the basis of the further addition of 0.8 v% jute fibers, the strength can still be enhanced by 20% and its thermal insulation properties will also be improved. Gradient design can further improve the mechanical properties of modified raw-soil-based wall materials and can weaken the loss of its inherent thermal insulation function.