Exploring advances in sulfur composite cathodes for lithium-sulfur batteries: A comprehensive review

Tiwari, Sakshi; Yadav, Venkteshwar; Poonia, A.K.; Pal, Dharm

doi:10.1016/j.est.2024.112347

Journal of Energy Storage

2024

DOI: 10.1016/j.est.2024.112347

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Exploring advances in sulfur composite cathodes for lithium-sulfur batteries: A comprehensive review

Sakshi Tiwari,

Venkteshwar Yadav,

A.K. Poonia

et al.

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Cited by 16 publications

References 108 publications

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Covalent Organic Frameworks and Their Derivatives for Applications in High‐Performance Lithium–Sulfur Batteries

Chen,

Jiang,

Liu

et al. 2024

Adv Funct Materials

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Lithium–Sulfur batteries (LSBs) are widely regarded as one of the most promising energy storage systems due to their ultra‐high theoretical energy density and environmental friendliness. However, practical applications of LSBs face significant challenges, including the shuttle effect of soluble polysulfides and the formation of lithium dendrites. Covalent organic frameworks (COFs) have emerged as potential materials for inhibiting the polysulfide shuttle effect and buffering lithium dendrites. This review provides an overview of the latest advancements in the use of COF and its derivative materials as sulfur host materials, modified commercial separators, and electrolytes in LBSs, and makes some brief conclusions and predictions. Pure COFs, COF derivatives, and COF composites are discussed as sulfur hosts, along with novel strategies intended to enhance LSB cycling stability and reversibility. Strategies for enhancing LSBs performance are summarized through the modification of separators using COFs, with the ultimate goal of achieving high energy density. It also discusses the strategies for designing COF‐based electrolytes, which include structural design, use of ionic COFs, and introduction of lithium salt molecules or flexible oligo(ethylene oxide) chains into COF skeletons. Additionally, the review discusses some future prospects for the use of COFs and their derivatives in LSBs.

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Covalent Organic Frameworks and Their Derivatives for Applications in High‐Performance Lithium–Sulfur Batteries

Chen,

Jiang,

Liu

et al. 2024

Adv Funct Materials

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Graphene-like porous carbon sheet/carbon nanotube composite as sulfur host for lithium-sulfur batteries

Fan,

Su,

et al. 2024

Ionics

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Utilization of Y-MOF-derived Y2O3/YS@C heterojunction for Li-S battery separators

Qian,

Xu,

Zhao

et al. 2025

Colloids and Surfaces A: Physicochemical and Engineering Aspect

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Exploring advances in sulfur composite cathodes for lithium-sulfur batteries: A comprehensive review

Cited by 16 publications

References 108 publications

Covalent Organic Frameworks and Their Derivatives for Applications in High‐Performance Lithium–Sulfur Batteries

Covalent Organic Frameworks and Their Derivatives for Applications in High‐Performance Lithium–Sulfur Batteries

Graphene-like porous carbon sheet/carbon nanotube composite as sulfur host for lithium-sulfur batteries

Utilization of Y-MOF-derived Y2O3/YS@C heterojunction for Li-S battery separators

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