This study aims to assess the potential benefits and barriers of Move to Flow (MtF), a nature-based physical activity (PA) programme structured in two levels that include movements related to the animal, vegetal, and inert nature. A questionnaire was applied to 133 participants from Spain, Latvia, and Serbia. The instrument was structured in the following sections: socio-economic variables; sports participation; and health and physical condition perception. In addition, the Exercise Benefits and Barriers Scale (EBBS), which assesses these aspects on the physical, psychological, and social levels, was included. Results showed that men aged 36–50 obtained the highest total and benefit scores, while women and the youngest scored higher in barriers. Data analysis shows associations between weekly engagement in physical activity and intensity (p < 0.001) and the perceived benefits of MtF. In the case of intensity, it is the same with barriers (p < 0.001). Similarly, there is an association between benefits and barriers and perceived health status (p < 0.001) and physical condition (p < 0.001). Furthermore, positive correlations were found in MtF between PA frequency, intensity, and health and physical condition (r = 0.755). In conclusion, this study has demonstrated MtF’s value as a cost-effective tool that empowers people to take an active role in improving their overall health and well-being.