2022
DOI: 10.1021/acsphotonics.1c01222
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Externally Driven Nonlinear Time-Variant Metasurfaces

Abstract: Resonant photonic nanostructures exhibiting enhanced nonlinear response and efficient frequency conversion are an emergent platform in nonlinear optics. High-index semiconductor metasurfaces with rapidly tuned high-quality-factor (high-Q) resonances enable a novel class of timevariant metasurfaces, which expands the toolbox of color management at the nanoscale. Here, we report on the dynamic control of the nonlinear optical response in time-variant semiconductor metasurfaces supporting high-Q resonances in the… Show more

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Cited by 19 publications
(7 citation statements)
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“…Recently, a blue-shift of the third-harmonic (TH) wavelength (also known as the photon acceleration effect) was observed in silicon metasurfaces supporting Mie resonances in the infrared range . This provides a direct way to control the dynamics of linear and nonlinear signals on the time scales comparable with or even less than the pulse length, as demonstrated in the recent experiments , with time-varying asymmetric metasurfaces. Self-action effects in metasurfaces with sharp resonances attract special attention because the strong field ionization regime can be realized even for moderate pump powers which in turn leads to an increase the mode line width of a high- Q resonance due to the generation of the electron–hole plasma in the material …”
mentioning
confidence: 72%
“…Recently, a blue-shift of the third-harmonic (TH) wavelength (also known as the photon acceleration effect) was observed in silicon metasurfaces supporting Mie resonances in the infrared range . This provides a direct way to control the dynamics of linear and nonlinear signals on the time scales comparable with or even less than the pulse length, as demonstrated in the recent experiments , with time-varying asymmetric metasurfaces. Self-action effects in metasurfaces with sharp resonances attract special attention because the strong field ionization regime can be realized even for moderate pump powers which in turn leads to an increase the mode line width of a high- Q resonance due to the generation of the electron–hole plasma in the material …”
mentioning
confidence: 72%
“…It poses limitations for the detection of scaled and rotated images and demands new techniques such as tunable metasurfaces. Electric, magnetic, , or photoinduced tuning of the metasurface optical response have been recently investigated. In the latter case, direct band gap semiconductors are promising materials, since optically tunable metasurfaces require significant modulation of the refractive index during carrier injection by a femtosecond laser pulse due to the bandfilling, bandgap shrinkage, and free-carrier absorption …”
Section: Discussionmentioning
confidence: 99%
“…[23] Linear frequency conversion is commonly interpreted from the temporal boundary of the real part of the refractive index, which is a straightforward analogy to the tone change of a guitar by adjusting string length after plucking. However, the dynamics in an unsteady photonic cavity with a subwavelength scale involves more complex processes, including the influence of correlated imaginary parts of the refractive index [24][25][26] and the intrinsic radiative and nonradiative losses of the cavity. The physics becomes nontrivial when all these factors are considered in the temporal boundary in practical scenarios.…”
Section: Introductionmentioning
confidence: 99%