Extreme ultraviolet time-resolved photoelectron spectroscopy of adenine, adenosine and adenosine monophosphate in a liquid flat jet

Koga, Masafumi; Kang, Do Hyung; Heim, Zachary N.; Meyer, Philipp; Erickson, Blake A.; Haldar, Neal; Baradaran, Negar; Havenith, Martina; Neumark, Daniel M.

doi:10.1039/d4cp00856a

Phys. Chem. Chem. Phys.

2024

DOI: 10.1039/d4cp00856a

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Extreme ultraviolet time-resolved photoelectron spectroscopy of adenine, adenosine and adenosine monophosphate in a liquid flat jet

Masafumi Koga,

Do Hyung Kang,

Zachary N. Heim

et al.

Abstract: Time-resolved photoelectron spectroscopy using an extreme-ultraviolet (XUV) probe pulse was used to investigate the UV photoinduced dynamics of adenine (Ade), adenosine (Ado), and adenosine-5-monophosphate (AMP) in a liquid water jet....

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Cited by 2 publications

References 103 publications

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Sub-20-fs UV-XUV beamline for ultrafast molecular spectroscopy

Crego,

Severino,

Mai

et al. 2024

Sci Rep

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We present an ultraviolet (UV) - extreme-ultraviolet (XUV) pump-probe beamline with applications in ultrafast time-resolved photoelectron spectroscopy. The UV pump pulses, tuneable between 255 and 285 nm and with µJ-level energy, are generated by frequency up-conversion between ultrashort visible/infrared pulses and visible narrow-band pulses. Few-femtosecond XUV probe pulses are produced by a high-order harmonic generation source equipped with a state-of-the-art time-delay compensated monochromator. Two-colour UV-XUV sidebands are used for a complete in situ temporal characterization of the pulses, demonstrating a temporal resolution of better than 20 fs. We validate the performances of the beamline through a UV-XUV pump-probe measurement on 1,3-cyclohexadiene, resolving the ultrashort dynamics of the first conical intersection. This instrument opens exciting possibilities for investigating ultrafast UV-induced dynamics of organic molecules in ultrashort time scales.

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Sub-20-fs UV-XUV beamline for ultrafast molecular spectroscopy

Crego,

Severino,

Mai

et al. 2024

Sci Rep

View full text Add to dashboard Cite

show abstract

Dynamics of photoexcited 5-bromouracil and 5-bromo-2′-deoxyuridine studied by extreme ultraviolet time-resolved photoelectron spectroscopy in liquid flat jets

Kang,

Koga,

Haldar

et al. 2024

Chem. Sci.

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Extreme ultraviolet time-resolved photoelectron spectroscopy of adenine, adenosine and adenosine monophosphate in a liquid flat jet

Abstract: Time-resolved photoelectron spectroscopy using an extreme-ultraviolet (XUV) probe pulse was used to investigate the UV photoinduced dynamics of adenine (Ade), adenosine (Ado), and adenosine-5-monophosphate (AMP) in a liquid water jet....

Cited by 2 publications

References 103 publications

Sub-20-fs UV-XUV beamline for ultrafast molecular spectroscopy

Sub-20-fs UV-XUV beamline for ultrafast molecular spectroscopy

Dynamics of photoexcited 5-bromouracil and 5-bromo-2′-deoxyuridine studied by extreme ultraviolet time-resolved photoelectron spectroscopy in liquid flat jets

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