Fabrication strategies for high-performance unbiased PEC water splitting cells

Ding, Lingling; Zhang, Yaqian; Wang, Tao; Li, Peng; Chang, Kun

doi:10.1039/d3cy01703f

Catal. Sci. Technol.

2024

DOI: 10.1039/d3cy01703f

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Fabrication strategies for high-performance unbiased PEC water splitting cells

Lingling Ding,

Yaqian Zhang,

Tao Wang

et al.

Abstract: Photoelectrochemistry (PEC) is an effective method for harvesting renewable hydrogen directly from water utilizing sunlight. Recent studies have shown that it is possible to achieve high solar-to-hydrogen (STH) using tandem-structured...

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Cited by 4 publications

References 161 publications

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Failure Mechanism Analysis and Emerging Strategies for Enhancing the Photoelectrochemical Stability of Photoanodes

Zhang,

Liu,

et al. 2024

ChemSusChem

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The development of efficient and stable photoanode materials is essential for driving the possible practical application of photoelectrochemical water splitting. This article begins with a basic understanding of the fundamentals of photoelectrochemical devices and photoanodes. State‐of‐the‐art strategies for designing photoanodes with long‐term stability are highlighted, including insertion of hole transport layers, construction of protective/passivation layers, loading of co‐catalysts, construction of heterojunctions, and modification of the electrolyte. Based on the insights gained from these effective strategies, we present an outlook for addressing key aspects of the challenges of stabilizing photoanodes development in the future work. Widespread adoption of stability assessment criteria will facilitate reliable comparisons of results from different laboratories. In addition, deactivation of photoanode is defined as a 50% reduction in productivity. An in‐depth understanding of the deactivation mechanism is essential for the design and development of efficient and stable photoanodes. This work will provide insights into the stability assessment of photoanode and facilitate the production of practical solar fuels.

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Failure Mechanism Analysis and Emerging Strategies for Enhancing the Photoelectrochemical Stability of Photoanodes

Zhang,

Liu,

et al. 2024

ChemSusChem

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BiVO4 photoanodes with enhanced photoelectrochemical performance: Preparation, modification and emerging applications

Wang,

Wan,

Feng

et al. 2025

Journal of Materials Science & Technology

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Enhanced charge separation of NiO/ZnO P-N heterojunction nanorod arrays for photoelectrochemical water splitting

Cai,

Tao,

Peng

et al. 2024

Surfaces and Interfaces

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Fabrication strategies for high-performance unbiased PEC water splitting cells

Abstract: Photoelectrochemistry (PEC) is an effective method for harvesting renewable hydrogen directly from water utilizing sunlight. Recent studies have shown that it is possible to achieve high solar-to-hydrogen (STH) using tandem-structured...

Cited by 4 publications

References 161 publications

Failure Mechanism Analysis and Emerging Strategies for Enhancing the Photoelectrochemical Stability of Photoanodes

Failure Mechanism Analysis and Emerging Strategies for Enhancing the Photoelectrochemical Stability of Photoanodes

BiVO4 photoanodes with enhanced photoelectrochemical performance: Preparation, modification and emerging applications

Enhanced charge separation of NiO/ZnO P-N heterojunction nanorod arrays for photoelectrochemical water splitting

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