Factorized time correlation diagram analysis of Raman induced Kerr effect spectroscopy using noisy light

Abstract

Articles you may be interested inLow-frequency collective dynamics in deep eutectic solvents of acetamide and electrolytes: A femtosecond Raman-induced Kerr effect spectroscopic study J. Chem. Phys. 141, 134506 (2014); 10.1063/1.4897207Isotropic and anisotropic Raman scattering from molecular liquids measured by spatially masked optical Kerr effect spectroscopy A combined instantaneous normal mode and time correlation function description of the optical Kerr effect and Raman spectroscopy of liquid CS 2The factorized time correlation ͑FTC͒ diagram analysis of Raman induced Kerr effect spectroscopy from noisy light is presented. The complete set of FTC diagrams is given. This process requires a more sophisticated FTC diagram analysis than is typical because of the important role color-locking plays for this spectroscopy. A physical understanding of the terms that give rise to the slow decaying asymmetric interferograms seen in the experimental literature can be gleaned from these FTC diagrams. The interferograms carry information about the decay of the librational coherences.

Two-Dimensional Electronic Spectroscopy Using Incoherent Light: Theoretical Analysis

“…To date, FTC diagram analysis has been applied to several noisy-light spectroscopies [113,[133][134][135][136] and also explored in a more general context [137,138] to elucidate the underlying mathematical structure of the diagrams. In all previous work the noisy-light signal was homodyne detected.…”

Polarized dressing suppression and enhancement involving Rydberg in a thermal vapor cell

“…The singly and doubly dressing theories are used to interpret the experimental results. Investigations of the interactions between SWM processes of Rydberg and non-Rydberg as well as their polarized dressing can help us to understand their underlying properties, which have many potential applications in nonlinear optics [21,22], quantum control [23], many-body interaction as well as inducing short-range interaction [24].…”