Multichannel calibration is essential for detecting moving targets and for estimating their positions and velocities accurately. This article presents a fast and efficient calibration algorithm for the along-track multichannel systems, in particular for space-time adaptive processing (STAP) techniques. The proposed algorithm corrects the phase and magnitude offsets of the receive channels and also takes into account the Doppler centroid variation (e.g., caused by atmospheric turbulences) along the slant range and the azimuth time. The knowledge of the Doppler centroid variation is especially important for an accurate clutter covariance matrix estimation, which is required by STAP for efficient clutter suppression. Important calibration parameters and offsets are estimated directly from the range-compressed training data. The proposed algorithm is evaluated based on real multichannel X-band radar data acquired with DLR's airborne system F-SAR and compared with the state-of-the-art digital channel balancing technique. The experimental results show the potential of the proposed calibration algorithm toward real-time applications.