Femtosecond-laser-induced spin-polarized electron emission from a GaAs tip

Abstract

It is shown that focusing circularly-polarized 800 nm light pulses of 100 fs duration on the tips of p-GaAs crystalline shards having no negative electron affinity (NEA) activation results in electron emission that is both fast and spin-polarized. The 400 fs duration of the emission process was determined by pump/probe measurements. The three samples we investigated produced electron polarizations of 13.1(9) %, 13.3(7) %, and 10.4(2) %. Emission currents ranged between 50 pA and 3 nA with a sample bias of −100 V and average laser power of 100 mW. The electron emission exhibited linear dichroism and was obtained under moderate vacuum conditions, similar to that of metallic tips. This source of spin-polarized electron pulses is "fast" in the sense that the electron emission process is of comparable duration to the laser pulses that initiate it.

Dependence of Ultrafast Electron Emission Characteristics of Graphene Cold Cathode on Femtosecond Photoexcitation Polarization Angle

“…Various ultrafast laser-excited mechanisms may contribute to the electron emission process, including photofield emission (PFE), , optical field emission (OFE) ,,− and multiphoton photoemission (MPP). − In this study, the PFE can be excluded initially, because the photon energy (∼1.55 eV) of excitation laser corresponding to 800 nm in wavelength is considerably less than the work function (∼4.5 eV) of the vFLGs cathode. Figure a also reveals a nonfield-induced characteristic as the vacuum gap electric field provided by the anode is too small (below 0.8 MV m –1 ) to turn on the electrostatic field emission.…”