2024
DOI: 10.1002/smll.202310224
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FeN3S1─OH Single‐Atom Sites Anchored on Hollow Porous Carbon for Highly Efficient pH‐Universal Oxygen Reduction Reaction

Shilong Zhou,
Chao Chen,
Jiawei Xia
et al.

Abstract: Regulating the asymmetric active center of a single‐atom catalyst to optimize the binding energy is critical but challenging to improve the overall efficiency of the electrocatalysts. Herein, an effective strategy is developed by introducing an axial hydroxyl (OH) group to the Fe─N4 center, simultaneously assisting with the further construction of asymmetric configurations by replacing one N atom with one S atom, forming FeN3S1─OH configuration. This novel structure can optimize the electronic structure and d‐… Show more

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Cited by 3 publications
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