Ferrorotational Selectivity in Ilmenites

Fang, Xiaochen; De, Chandan; Huang, Fei-Ting; Xu, Xianghan; Du, Kai; Wang, Kefeng; Li, Bingqing; Cheong, Sang-Wook

doi:10.1021/jacs.3c08635

J. Am. Chem. Soc.

2023

DOI: 10.1021/jacs.3c08635

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Ferrorotational Selectivity in Ilmenites

Xiaochen Fang,

Chandan De,

Fei-Ting Huang

et al.

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Cited by 5 publications

References 39 publications

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Conversion between dipoles with different spatial parities by circularly polarized light

Hayami

2025

Materials Today Quantum

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Conversion between dipoles with different spatial parities by circularly polarized light

Hayami

2025

Materials Today Quantum

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Emergence of chirality from electron spins, physical fields, and material-field composites

Kusunose,

Kishine,

Yamamoto

2024

Applied Physics Letters

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In this work, chirality in spin-active electronic states is explained clearly to address confusion about chiral effects recently discovered in materials science. We stress that the electronic toroidal monopole G0 can serve as a measure of chirality. By using the symmetry classification in terms of four distinct types of multipole bases, we extend the concept of chirality from materials to physical fields and material-field composites. Additionally, we illustrate specific examples from physics and chemistry that demonstrate the process of acquiring chirality through the combination of seemingly achiral degrees of freedom, which we term the emergence of chirality. Interference between multiple chiralities exhibiting phenomena specific to handedness is also discussed.

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Optical control of ferroaxial order

He,

Khalsa

2024

Phys. Rev. Research

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Materials that exhibit ferroaxial order hold potential for novel multiferroic applications. However, in pure ferroaxials, domains are not directly coupled to stress or static electric field due to their symmetry, limiting the ability to pole and switch between domains—features required for real-world applications. Here we propose a general approach to selectively condense and switch between ferroaxial domains with light. We show that circularly polarized light pulses on resonance with infrared-active phonons manifest helicity-dependent control over ferroaxial domains. Nonlinear contributions to the lattice polarizability play an essential role in this phenomenon. We illustrate the feasibility of our approach using first-principles calculations and dynamical simulations for the archetypal ferroaxial material RbFe(MoO4)2. Our results are discussed in the context of future pump-probe optical experiments, where polarization, carrier frequency, and fluence threshold are explored. Published by the American Physical Society 2024

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Ferrorotational Selectivity in Ilmenites

Cited by 5 publications

References 39 publications

Conversion between dipoles with different spatial parities by circularly polarized light

Conversion between dipoles with different spatial parities by circularly polarized light

Emergence of chirality from electron spins, physical fields, and material-field composites

Optical control of ferroaxial order

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