Field trial of hollow fiber modules of hybrid facilitated transport membranes for flue gas CO2 capture in cement industry

Janakiram, Saravanan; Fabio, Santinelli; Costi, Riccardo; Lindbråthen, Arne; Nardelli, Giuseppe Marino; Milkowski, Kris; Ansaloni, Luca; Deng, Liyuan

doi:10.1016/j.cej.2020.127405

Cited by 43 publications

(22 citation statements)

References 45 publications

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“…The performance selected are similar to materials reported by other research groups that have already reached pilot scale [31]. FTMs have already been demonstrated in flue gas from cement plants with good stability over time even in the presence of impurities [23][24][25]. A single stage configuration is considered for the separation as shown in Figure 2.…”

Section: Facilitated Transport Membranesmentioning

confidence: 61%

“…These results indicate a clear direction for material development that should aim at increasing the performance at a reduced humidity content, but maintaining the high selectivity ensured by the facilitated transport mechanism. Pre-pilot tests in situ showed how the membranes could operate with a reduced humidity but with lower performances [24,25].…”

Section: Comparison With Other Capture Technologiesmentioning

confidence: 99%

“…A first generation of these materials was already tested in a cement plant in Norway by prof. Hagg et al [23] with promising results and a prediction of a significant reduction in the cost of capture if improved CO 2 permeance was achieved. The new materials evaluated in this study were produced in the framework of the Horizon2020 funded project NANOMEMC 2 and evaluated for a specific site in Gubbio, Italy where the materials were also tested experimentally [24,25].…”

Section: Introductionmentioning

confidence: 99%

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Assessment on the Application of Facilitated Transport Membranes in Cement Plants for CO2 Capture

Ferrari

Amelio

Nardelli³

et al. 2021

Energies

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Carbon dioxide capture from cement plant flue gas can play an important role in mitigating CO2 emission that lead to climate change. Among all the technologies evaluated, membranes have potential to be one of the most energy-efficient and low-cost CO2 capture option. In this work, a novel membrane technology, Facilitated Transport Membranes (FTMs), is assessed to further reduce energy demand and cost for CO2 capture in a cement plant. A new process that employs FTMs is simulated and applied to a real clinker production plant in Italy (Colacem, Gubbio). The process is then compared with other carbon capture technologies. Results show that the FTM technology can be competitive with other technologies despite the need of steam to operate the membrane. Despite the benefit in terms of specific emission compared to more established absorption with liquid amines process, further improvements on membrane performances are needed to gain also an economic advantage for carbon capture in the cement industry.

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Section: Facilitated Transport Membranesmentioning

confidence: 61%

Section: Comparison With Other Capture Technologiesmentioning

confidence: 99%

Section: Introductionmentioning

confidence: 99%

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Assessment on the Application of Facilitated Transport Membranes in Cement Plants for CO2 Capture

Ferrari

Amelio

Nardelli³

et al. 2021

Energies

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“…The pilot field trials include the Norwegian University of Science and Technology (NTNU) and SINTEF’s tests at the SINTEF Tiller plant (Trondheim, Norway) [ 52 ], the Norcem cement factory (Brevik, Norway) [ 53 ], the Colacem cement plant (Gubbio, Italy) [ 54 , 55 ], and the Sines bituminous coal power station (Sines, Portugal) [ 56 ]. Helmholtz-Zentrum Geesthacht (HZG) has also undertaken a field test at a hard coal power station (Baden-Württemberg, Germany) [ 57 ], while the Cooperative Research Centre for Greenhouse Gas Technologies (CO2CRC) and the University of Melbourne (UM) have conducted their membrane separation trial at a lignite-fired power station (Victoria, Australia) [ 58 ].…”

Section: Membrane Scale-up Modular Fabrication and Field Testsmentioning

confidence: 99%

“…Compared with the previous membrane containing the mobile carrier, new facilitated transport HF membranes were synthesized by NTNU by incorporating sterically hindered polyallylamine [ 55 ]. 200-cm 2 HF modules were also tested at the Colacem cement plant.…”

Section: Membrane Scale-up Modular Fabrication and Field Testsmentioning

confidence: 99%

Recent Progress in the Engineering of Polymeric Membranes for CO2 Capture from Flue Gas

Han

Yang

2020

Membranes

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CO2 capture from coal- or natural gas-derived flue gas has been widely considered as the next opportunity for the large-scale deployment of gas separation membranes. Despite the tremendous progress made in the synthesis of polymeric membranes with high CO2/N2 separation performance, only a few membrane technologies were advanced to the bench-scale study or above from a highly idealized laboratory setting. Therefore, the recent progress in polymeric membranes is reviewed in the perspectives of capture system energetics, process synthesis, membrane scale-up, modular fabrication, and field tests. These engineering considerations can provide a holistic approach to better guide membrane research and accelerate the commercialization of gas separation membranes for post-combustion carbon capture.

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Modified COSMO‐UNIFAC model for ionic liquid–CO₂ systems and molecular dynamic simulation

Zhu

Gui

et al. 2022

AIChE Journal

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A new predictive molecular thermodynamic model (i.e., modified COSMO-SAC-UNIFAC) was first proposed and extended to predict the solubility of CO 2 in pure and mixed ionic liquids (ILs) at the temperatures down to 263.2 K. It is interesting to discover that with equimolar amounts, the solubility of CO 2 in such 1:was consistent at the same temperature and pressure in the case of exchanging their respective cations and anions. The molecular dynamic (MD) simulation for CO 2 + mixed ILs was performed to deeply analyze and explain this intriguing phenomenon. Not only the CO 2 gas drying experiment with the ILs ([C2mim][OAc], [C2mim][dca], and [C2mim][OAc] + [C2mim][dca])as absorbents but also the corresponding process simulation and optimization were made to stress the effectiveness and applicability of the new thermodynamic model.

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Field trial of hollow fiber modules of hybrid facilitated transport membranes for flue gas CO2 capture in cement industry

Cited by 43 publications

References 45 publications

Assessment on the Application of Facilitated Transport Membranes in Cement Plants for CO2 Capture

Assessment on the Application of Facilitated Transport Membranes in Cement Plants for CO2 Capture

Recent Progress in the Engineering of Polymeric Membranes for CO2 Capture from Flue Gas

Modified COSMO‐UNIFAC model for ionic liquid–CO₂ systems and molecular dynamic simulation

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Field trial of hollow fiber modules of hybrid facilitated transport membranes for flue gas CO2 capture in cement industry

Cited by 43 publications

References 45 publications

Assessment on the Application of Facilitated Transport Membranes in Cement Plants for CO2 Capture

Assessment on the Application of Facilitated Transport Membranes in Cement Plants for CO2 Capture

Recent Progress in the Engineering of Polymeric Membranes for CO2 Capture from Flue Gas

Modified COSMO‐UNIFAC model for ionic liquid–CO2 systems and molecular dynamic simulation

Contact Info

Product

Resources

About

Modified COSMO‐UNIFAC model for ionic liquid–CO₂ systems and molecular dynamic simulation