Abstract. Located in the world's “third pole” and a remote region
connecting the Indian plate and the Eurasian plate, Qomolangma National
Nature Preserve (QNNP) is an ideal region to study the long-range transport
of atmospheric pollutants. In this study, gaseous elemental mercury (GEM),
gaseous oxidized mercury (GOM) and particle-bound mercury (PBM) were
continuously measured during the Indian monsoon transition period in QNNP. A
slight increase in the GEM concentration was observed from the period preceding the
Indian summer monsoon (1.31±0.42 ng m−3) to the Indian
summer monsoon period (1.44±0.36 ng m−3), while significant
decreases were observed in the GOM and PBM concentrations, with concentrations
decreasing from 35.2±18.6 to 19.3±10.9 pg m−3 (p < 0.001) for GOM and from 30.5±12.5 to 24.9±19.8 pg m−3
(p < 0.001) for PBM. A unique daily pattern was
observed in QNNP with respect to the GEM concentration,
with a peak value before sunrise and a low value at noon.
Relative to the (low) GEM concentrations, GOM concentrations (with a mean value
of 21.4±13.4 pg m−3, n=1239) in this region were relatively
high compared with the measured values in some other regions of China. A
cluster analysis indicated that the air masses transported to QNNP changed
significantly at different stages of the monsoon, and the major potential mercury
(Hg) sources shifted from northern India and western Nepal to eastern Nepal and Bangladesh.
As there is a large area covered in glaciers in QNNP, local glacier
winds could increase the transboundary transport of pollutants and transport
polluted air masses to the Tibetan Plateau. The atmospheric Hg concentration
in QNNP in the Indian summer monsoon period was influenced by transboundary
Hg flows. This highlights the need for a more specific identification of Hg
sources impacting QNNP and underscores the importance of international
cooperation regarding global Hg controls.