Fischer-Tropsch to olefin reaction over Fe-based catalysts: Effect of preparation method and synergistic effect of Mn and Zr promoters

Akbari, Maryam; Mirzaei, Ali Akbar

doi:10.1016/j.jtice.2024.105484

Journal of the Taiwan Institute of Chemical Engineers

2024

DOI: 10.1016/j.jtice.2024.105484

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Fischer-Tropsch to olefin reaction over Fe-based catalysts: Effect of preparation method and synergistic effect of Mn and Zr promoters

Maryam Akbari,

Ali Akbar Mirzaei

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Cited by 2 publications

References 96 publications

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Features of the behavior of nanosized catalytic dispersions in Fischer-Tropsch synthesis in slurry reactors of the CSTR and SBCR types

Kuzmin,

Dementieva,

Kulikova

et al. 2025

Journal of the Taiwan Institute of Chemical Engineers

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Features of the behavior of nanosized catalytic dispersions in Fischer-Tropsch synthesis in slurry reactors of the CSTR and SBCR types

Kuzmin,

Dementieva,

Kulikova

et al. 2025

Journal of the Taiwan Institute of Chemical Engineers

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Effect of the Reactor Material on the Reforming of Primary Syngas

Bezerra Silva,

Lugo-Pimentel,

Ceballos

et al. 2024

Molecules

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Syngas, mostly hydrogen and carbon monoxide, has traditionally been produced from coal and natural gas, with biomass gasification later emerging as a renewable process. It is widely used in fuel synthesis through the Fischer–Tropsch (FT) process, where the H2/CO ratio is crucial in determining product efficiency and quality. In this sense, this study aimed to reform an emulated syngas resulting from the supercritical water gasification of biomass, tailoring it to meet the H2/CO ratio required for FT synthesis. Conditions resembling dry reforming were applied, using temperatures from 600 to 950 °C and steel wool as a catalyst. Additionally, the effects of Inconel and stainless steel as reactor materials on syngas reforming were investigated. When Inconel was used, H2/CO ratios ranged between 1.04 and 1.84 with steel wool and 1.28 and 1.67 without. When comparing reactions without steel wool performed either in the Inconel or the stainless steel reactors, those using Inconel consistently outperformed the stainless steel ones, achieving CH4 and CO2 conversions up to 95% and 76%, respectively, versus 0% and 39% with stainless steel. It was concluded that the Inconel reactor exhibited catalytic properties due to its high nickel content and specific oxides.

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Fischer-Tropsch to olefin reaction over Fe-based catalysts: Effect of preparation method and synergistic effect of Mn and Zr promoters

Cited by 2 publications

References 96 publications

Features of the behavior of nanosized catalytic dispersions in Fischer-Tropsch synthesis in slurry reactors of the CSTR and SBCR types

Features of the behavior of nanosized catalytic dispersions in Fischer-Tropsch synthesis in slurry reactors of the CSTR and SBCR types

Effect of the Reactor Material on the Reforming of Primary Syngas

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