Floatable S-scheme Bi2WO6/C3N4/carbon fiber cloth composite photocatalyst for efficient water decontamination

Cai, Mingjie; Liu, Yanping; Dong, Kexin; Chen, Xiaobo; Li, Shijie

doi:10.1016/s1872-2067(23)64496-1

Cited by 174 publications

(11 citation statements)

References 78 publications

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“…In general, a smaller semicircle radius indicates a stronger charge transfer ability. 55 When compared with pure ZnO and MoS 2 , MZ-15 exhibits a smaller EIS Nyquist arc radius. 56 This obviously shows that the combination of ZnO and MoS 2 is beneficial for reducing the resistance of the nanocomposite, and improving the transfer efficiency of photogenerated carriers.…”

Section: Resultsmentioning

confidence: 94%

Highly efficient degradation of tetracycline by activated peroxymonosulfate over MoS₂/ZnO heterostructure nanocomposites

Jiang,

Wang,

Zhou

et al. 2023

New J. Chem.

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Section: Resultsmentioning

confidence: 94%

Highly efficient degradation of tetracycline by activated peroxymonosulfate over MoS₂/ZnO heterostructure nanocomposites

Jiang,

Wang,

Zhou

et al. 2023

New J. Chem.

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“…For starters, CoMo-LDHs were grown on a carbon cloth (CC) substrate via a simple binderless autocatalytic growth approach. The CC substrate has the potential to enhance electrical conductivity, encourage electron transfer, and enhance both catalytic efficiency and endurance . Urea releases OH – and CO2–3 ions in hydrothermal processes, which facilitate the formation of CoMo-LDHs.…”

Section: Resultsmentioning

confidence: 99%

“…However, the unsatisfactory conductivity of these materials limits their further development. To solve the above dilemma, heterojunction fabrication has emerged as a reasonable approach. − The construction of heterogeneous bimetallic selenides provides abundant phase boundaries and better conductivity. Notably, heterogeneous bimetal selenides could minimize the activation energy, and expedite the reaction kinetics, thereby refining their electrochemical ability by enhancing charge transport through the adjustment of charge at the heterogeneous interface. , For example, Bose et el.…”

Section: Introductionmentioning

confidence: 99%

Three-Dimensional Heterostructured CoSe₂/MoSe₂@CC as Trifunctional Electrocatalysts for Energy-Efficient Hydrogen Production

Yang,

Xiong,

Yang

et al. 2024

Energy Fuels

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Electrochemical water cracking to hydrogen production is a key technology for storing and converting energy. However, the energy consumption of this method comes mainly from the slow anodic oxygen evolution reaction (OER). Replacement of the OER with the urea oxidation reaction (UOR) enables energyefficient hydrogen production, avoiding dangerous H 2 /O 2 mixtures due to the release of N 2 and CO 2 at the anode. Hence, it is crucial to investigate efficient multifunctional electrocatalysts to assist OER in combination with hydrogen evolution reaction (HER) in improving the energy efficiency of hydrogen production. In this work, we take a feasible strategy to synthesize three-dimensional (3D) highly active catalysts CoSe 2 / MoSe 2 grown on carbon cloth (CoSe 2 /MoSe 2 @CC). Taking advantage of synergistic interaction between interfaces, CoSe 2 /MoSe 2 @CC exhibits a promising overpotential of 71 and 320 mV for HER and OER at 10 mA cm −2 , respectively. In addition, CoSe 2 / MoSe 2 @CC-4 also showed prominent catalytic activity against UOR in 1 M KOH with 0.3 M urea. An electrolyzer is also constructed via using CoSe 2 /MoSe 2 @CC as both electrodes. It is worth mentioning that the electrolyzer CoSe 2 /MoSe 2 @CC∥CoSe 2 /MoSe 2 @CC in 1 M KOH with 0.3 M urea obtains a battery voltage of 1.48 V to generate a current density of 10 mA cm −2 , which is 0.17 V lower than that in 1 M KOH (1.65). This electrolyzer completed relatively conspicuous durability in an alkaline electrolyte solution of 1 M KOH, with maintenance of initial current density through 24 h of continuous operation at a constant cell voltage for water splitting. This work develops a promising multifunctional catalyst for urea-assisted hydrogen generation from water electrolysis, which can reduce the decomposition potential of water electrolysis.

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“…Z‐scheme (or S‐scheme) composites facilitate charge transfers that emulate natural photosynthetic processes, fostering optimal electron and hole transport to dramatically curtail charge recombination. [ 54–59 ] Analogous to semiconductor‐semiconductor composites, Z‐scheme composites can incorporate semiconductors with diverse bandgaps for expanded light absorption. Yet, crafting an efficacious Z‐scheme system necessitates a comprehensive grasp of the associated semiconductors and their energetics.…”

Section: Synthesis and Optimizationmentioning

confidence: 99%

Photocatalytic Fibers for Environmental Purification: Challenges and Opportunities in the Post‐Pandemic Era

Wu,

Chen,

Chien

et al. 2023

Adv Energy and Sustain Res

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The COVID‐19 pandemic has underscored the paramount importance of maintaining clean and safe environments. Strengthening environmental purification measures is pivotal for better preparedness and resilience against future health crises. Photocatalytic fibers, due to their versatility and adaptability to various application scenarios, play a pivotal role in the field of environmental purification. In this perspective, light is shed on the pivotal advancements in employing photocatalytic fibers to tackle environmental issues encompassing dye degradation, antibiotics decomposition, heavy metal removal, indoor air purification, and microbial disinfection. These applications hold significant promise in promoting cleaner and healthier environments while aligning with sustainability objectives. However, the implementation of photocatalytic fibers in practical scenarios is not without its challenges. Issues, such as near infrared responsiveness, all‐day active capacity, reusability, and scalability, must be addressed to ensure their reliability and long‐term effectiveness. Potential solutions for surmounting these challenges are also delved, aiming to provide a comprehensive overview for researchers and stakeholders. Exploring new avenues and innovative approaches may pave the way for the widespread deployment of photocatalytic fibers in environmental purification, especially in the post‐pandemic era where the need for clean and safe environments is more evident than ever.

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Floatable S-scheme Bi2WO6/C3N4/carbon fiber cloth composite photocatalyst for efficient water decontamination

Cited by 174 publications

References 78 publications

Highly efficient degradation of tetracycline by activated peroxymonosulfate over MoS₂/ZnO heterostructure nanocomposites

Highly efficient degradation of tetracycline by activated peroxymonosulfate over MoS₂/ZnO heterostructure nanocomposites

Three-Dimensional Heterostructured CoSe₂/MoSe₂@CC as Trifunctional Electrocatalysts for Energy-Efficient Hydrogen Production

Photocatalytic Fibers for Environmental Purification: Challenges and Opportunities in the Post‐Pandemic Era

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Floatable S-scheme Bi2WO6/C3N4/carbon fiber cloth composite photocatalyst for efficient water decontamination

Cited by 174 publications

References 78 publications

Highly efficient degradation of tetracycline by activated peroxymonosulfate over MoS2/ZnO heterostructure nanocomposites

Highly efficient degradation of tetracycline by activated peroxymonosulfate over MoS2/ZnO heterostructure nanocomposites

Three-Dimensional Heterostructured CoSe2/MoSe2@CC as Trifunctional Electrocatalysts for Energy-Efficient Hydrogen Production

Photocatalytic Fibers for Environmental Purification: Challenges and Opportunities in the Post‐Pandemic Era

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Product

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About

Highly efficient degradation of tetracycline by activated peroxymonosulfate over MoS₂/ZnO heterostructure nanocomposites

Highly efficient degradation of tetracycline by activated peroxymonosulfate over MoS₂/ZnO heterostructure nanocomposites

Three-Dimensional Heterostructured CoSe₂/MoSe₂@CC as Trifunctional Electrocatalysts for Energy-Efficient Hydrogen Production