Biaxially textured REBa2Cu3–xCoxO7–z (RE = Gd,Y) films were prepared on (00l) LaAlO3 substrate using self‐developed fluorine‐free chemical solution deposition (CSD) approach. The in‐field Jc values are significantly improved for REBa2Cu3–xCoxO7–z films through low‐level Co doping. Co‐doped GdBa2Cu3O7–z film shows the highest Jc values at higher temperatures and fields, whereas the Jc values of Co‐doped YBa2Cu3O7–z film surpass that of other films at lower temperatures and fields. In addition, the volume pinning force densities of films with Co doping have been distinctly enhanced in the applied fields, indicating improved flux‐pinning properties. The possible reasons are discussed in detail.