Flame spectra within the UV/visible-light range are measured for a turbulent, liquid-fueled, swirl-stabilized, leandirect injection combustor. The flame spectra are quite similar to those of lean premixed combustion, which can be attributed to the small droplet size and fast fuel/air mixing. Broadband background emissions around 431 nm, which mainly consist of CO 2 chemiluminescence, are found to be self-similar with wavelength for both stable and unstable combustion. Chemiluminescence from OH , CH , and CO 2 is found to be a nonlinear function of the airflow rate, the equivalence ratio, preheat temperature, and pressure. Procedures for the determination of the instantaneous heat release rate and equivalence ratios along the flame front are developed. For both combustion instability and forced flame responses, the prediction errors are within 2.0% in the mean heat release rate, the mean air consumption rate, and the mean equivalence ratio. The assumption that chemiluminescence is proportional to the instantaneous heat releaser rate is generally invalid. Probably the proportionality is valid only in the weakly turbulent or wrinkled flamelet region in the absence of equivalence ratio variations and strong acoustic oscillations.
NomenclatureCHs = Laplace transform of CH chemiluminescence It = instantaneous chemiluminescence intensity, AU L f = curvilinear flame front _ m a t = instantaneous air consumption rate, g=s _ m a t = instantaneous air consumption rate divided by 100 g=s pt = instantaneous combustor pressure divided by the atmospheric pressure p 0 a t = acoustic pressure near the heat release zone, Pa p f t = instantaneous fuel pressure 0.29 m upstream of the fuel nozzle, Pa _ Q R t = instantaneous heat release rate, kW S L = laminar burning velocity, m=s s = symbol of the Laplace transform T = mean temperature in the heat release zone, K T 0 a t = acoustic temperature near the heat release zone, K T i = preheat temperature, K Xs = Laplace transform of xt jWsj = gain of the transfer function Ws Ws = phase angle of the transfer function Ws, deg = thermal diffusivity, m 2 =s H R = lower heating value of fuel, J=kg L = thickness of the laminar flame, m = fuel/air equivalence ratio = wave length divided by 431 nm = wavelength, nm a = air density, kg=m 3 u = reactant density, kg=m 3 c = chemical reaction time, s