The exposure of Mediterranean forests to large wildfires requires mechanisms to prevent and mitigate their negative effects on the territory and ecosystems. Fuel models synthesize the complexity and heterogeneity of forest fuels and allow for the understanding and modeling of fire behavior. However, it is sometimes challenging to define the fuel type in a structurally heterogeneous forest stand due to the mixture of characteristics from the different types and limitations of qualitative field observations and passive and active airborne remote sensing. This can impact the performance of classification models that rely on the in situ identification of fuel types as the ground truth, which can lead to a mistaken prediction of fuel types over larger areas in fire prediction models. In this study, a handheld mobile laser scanner (HMLS) system was used to assess its capability to define Prometheus fuel types in 43 forest plots in Aragón (NE Spain). The HMLS system captured the vertical and horizontal distribution of fuel at an extremely high resolution to derive high-density three-dimensional point clouds (average: 63,148 points/m2), which were discretized into voxels of 0.05 m3. The total number of voxels in each 5 cm height stratum was calculated to quantify the fuel volume in each stratum, providing the vertical distribution of fuels (m3/m2) for each plot at a centimetric scale. Additionally, the fuel volume was computed for each Prometheus height stratum (0.60, 2, and 4 m) in each plot. The Prometheus fuel types were satisfactorily identified in each plot and were compared with the fuel types estimated in the field. This led to the modification of the ground truth in 10 out of the 43 plots, resulting in errors being found in the field estimation between types FT2–FT3, FT5–FT6, and FT6–FT7. These results demonstrate the ability of the HMLS systems to capture fuel heterogeneity at centimetric scales for the definition of fuel types in the field in Mediterranean forests, making them powerful tools for fuel mapping, fire modeling, and ultimately for improving wildfire prevention and forest management.