“…From the early stage of tens of percent level energy spread and few mm mrad-level emittance, LWFA electron beams have now achieved electron beams with nC-level charge [4,5] , few per-mille-level relative energy spread [6][7][8][9] and sub-mm mrad-level emittance [10] . Benefitted from the ultra-high acceleration gradient of LWFA [11][12][13][14][15] , ultracompact radiation sources, such as betatron radiation [16][17][18] , Compton scattering [19][20][21][22] and tabletop free electron lasers (FELs) [23][24][25] , injectors for future colliders [26] will be possible. Most LWFA-based applications require an excellent 6D electron beam brightness [27,28] , defined by B 6D = I P ε nx ε ny σ γ •0.1% , where I P is the peak current, σ γ is the relative energy spread and ε nx and ε ny are the normalized Correspondence to: Ke Feng, Wentao Wang, and Ruxin Li, State Key Laboratory of High Field Laser Physics and CAS Center for Excellence in Ultra-intense Laser Science, Shanghai Institute of Optics and Fine Mechanics (SIOM), Chinese Academy of Sciences (CAS), Shanghai 201800, China.…”