including microelectromechanical (MEMS) actuators, [8][9][10][11][12] microscale heat exchangers, [13,14] soft and wearable electronics, [15][16][17][18][19] and reconfigurable structures. [20,21] Several techniques have been developed to control the motion and deformation of liquid metal droplets. Applying an external potential gradient is the most commonly used method to drive and deform liquid metal within electrolytes. [8,9,12,22] Other approaches for driving liquid metal droplets by inducing chemical reactions, [23,24] and ionic imbalance [25] have also been demonstrated. Recently, the actuation of liquid metal droplets using external magnetic fields has been explored through the modification of liquid metal surface with ferromagnetic materials. For example, liquid metal coated with iron (Fe) nanoparticles (NPs) can be manipulated, merged, and separated in microfluidic channels with various angles in discretionary direction using an external magnetic field. [26] Other ferromagnetic materials such as nickel can be electroplated on the surface of liquid metal to form a motor. [27] The liquid metal motor can be controlled using both magnetic and electric fields, and also can achieve autonomous locomotion by reacting with aluminum foil. Similarly, porous structure of liquid metal can be obtained by mixing liquid metal and iron NPs in hydrochloric acid. [28] Such a porous mix can expand when subjected to heating to control its density. However, the above-mentioned approaches using electroplating or NP coating/mixing significantly affect the intrinsic properties of liquid metal and may sacrifice the surface fluidity, deformability, and flexibility of the material.Gallium-based room temperature liquid metal alloys have recently been explored to be an emerging functional material. They have attracted particular attentions in a variety of applications due to their unique properties. Many of the applications are based on the precise control over the motion of liquid metal, and yet, the fact that currently lacking the advanced and reliable controlling methods greatly hinders the potential of liquid metal to be applied in a wider range of fields. In this study, an innovative approach is developed to obtain functional liquid metal (FLM) by modifying it with copper-iron magnetic nanoparticles (Cu-Fe NPs). The magnetic modification process enables the Cu-Fe NPs to be suspended within the liquid metal and form the FLM. The FLM exhibits similar appearance, actuating behaviors, and deformability in alkaline solutions to those of pure liquid metal alloys. Meanwhile, the magnetic modification enables the precise and rapid manipulation of the liquid metal using a magnetic field. Most importantly, for the first time, the precise control and climbing locomotion of the FLM is demonstrated with the interworking of both electric and magnetic fields simultaneously. The remarkable features of the FLM may represent vast potentials toward the development of future intelligent soft robots.