2009
DOI: 10.1103/physrevb.80.045324
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From quantum dots to quantum wires: Electronic structure of semiconductor nanorods

Abstract: The transition bridge between zero-dimensional quantum dots and one-dimensional quantum wires is explored theoretically by means of the construction of the addition energy spectra of nanorods with different lengths. Spin density-functional theory supplemented with full configuration interaction calculations are carried out. The addition energy spectra are qualitatively related to the single particle correlation diagram. The transition from charge-density waves to spin-density waves, characterizing the Wigner c… Show more

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Cited by 22 publications
(12 citation statements)
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“…Therefore, a more general description is needed in order to take subband mixing into account. Quantitatively exact modeling of such nontrivial optical properties of nanostructures must be based on atomistic or multi-band kp methods [10,12]. However, it may be useful and interesting to have a simple semi-quantiative model that would not only elucidate the physical mechanism of the polarization but also yield an estimate of the expected effect in terms of the shape parameters.In this contribution, we present a "minimal" theory that is able to account for the observed DOP in the QDash luminescence.…”
mentioning
confidence: 99%
“…Therefore, a more general description is needed in order to take subband mixing into account. Quantitatively exact modeling of such nontrivial optical properties of nanostructures must be based on atomistic or multi-band kp methods [10,12]. However, it may be useful and interesting to have a simple semi-quantiative model that would not only elucidate the physical mechanism of the polarization but also yield an estimate of the expected effect in terms of the shape parameters.In this contribution, we present a "minimal" theory that is able to account for the observed DOP in the QDash luminescence.…”
mentioning
confidence: 99%
“…The FCI program used is the same as in Ref. 27. As in such a paper, a basis set ensuring saturation along the NR axis is employed.…”
Section: Methods Validation and Illustrative Calculationsmentioning
confidence: 99%
“…The transition to the Fermi liquid goes through an intermediate phase, called charge-density wave ͑CDW͒,with N / 2 peaks in the density profile. 2,[11][12][13] This phase may also be considered as a partially melted Wigner molecule.…”
Section: Introductionmentioning
confidence: 99%
“…In a recent paper, 13 we theoretically studied, within the local spin-density-functional theory ͑LSDFT͒, the electronic structure of nanorods ͑NRs͒, elongated QDs which constitute the bridge between zero-dimensional QDs and one-dimensional quantum wires ͑QWs͒, and monitorized the Wigner crystallization in the addition energy spectra. Note that, by changing the gate voltage attached to a nanocrystal, tunnel conductance and capacitance measures yield a peak every time the number of electrons in the QD increases by one.…”
Section: Introductionmentioning
confidence: 99%