2017
DOI: 10.1103/physrevb.96.224427
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Frustrated antiferromagnetic honeycomb-tunnel-like latticeCuR2Ge2O8(R=Pr, Nd, S

Abstract: New frustrated antiferromagnetic compounds CuRE2Ge2O8 (RE=Pr, Nd, Sm, Eu) have been investigated using high-resolution x-ray diffraction, magnetic and heat capacity measurements. These systems show different magnetic lattices depending on rare-earth element. The nonmagnetic Eu compound is a S=1/2 two-dimensional triangular antiferromagnetic lattice oriented in the ac plane with geometrical frustration. On the other hand, the Pr, Nd, and Sm compounds show a threedimensional honeycomb-tunnel-like lattice made of… Show more

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Cited by 8 publications
(7 citation statements)
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“…There are many experimental works dedicated to the frustrated spin systems where they were studied by means of optical second-harmonic spectroscopy, measurements of magnetization, susceptibility and specific heat, resistivity measurements, synchrotron X-rays and neutron diffraction, Mössbauer technique etc. [1,2,3,4,5,6,7,8,9,10,11,12,13,14,15,16,17,18,19,20,21,22,23]. The results of these experiments turn out to be rather contradictory.…”
Section: Introductionmentioning
confidence: 96%
“…There are many experimental works dedicated to the frustrated spin systems where they were studied by means of optical second-harmonic spectroscopy, measurements of magnetization, susceptibility and specific heat, resistivity measurements, synchrotron X-rays and neutron diffraction, Mössbauer technique etc. [1,2,3,4,5,6,7,8,9,10,11,12,13,14,15,16,17,18,19,20,21,22,23]. The results of these experiments turn out to be rather contradictory.…”
Section: Introductionmentioning
confidence: 96%
“…Because the negative thermal expansion is expected to occur in the antiferromagnetic phase near the boundary to the ferromagnetic phase, the solid solution system is promising because the strength ratio |J FM |/J AF can be tuned rather continuously by varying the Zn concentration. In addition to the honeycomb-lattice antiferromagnets, magnets having edge-sharing M X 6 octahedra also provide candidate materials [57][58][59][60][61][62][63]. We expect that the present work will contribute to diversify the family of materials hosting the magnetism-induced negative thermal expansion.…”
Section: Conclusion and Discussionmentioning
confidence: 99%
“…The present work provides an important guiding principle for the material search and will diversify the family of materials hosting the negative thermal expansion. There are a huge number of honeycomb lattice transition-metal compounds which exhibit antiferromagnetic and ferrimagnetic [53][54][55][56] phases or related crystal structures [57][58][59][60][61][62][63]. These compounds are candidate hosts of the magnetism-driven negative thermal expansion based on the proposed mechanism.…”
Section: Introductionmentioning
confidence: 99%
“…Finding these parameters along with critical exponents for such chiral universality class had given contradictory results in field-theoretical models compared to experiments [29,30]. Also the results of different experiments had produced a wide range of unrelated critical exponents and even the order of phase transition was found to differ for materials with same symmetry [31,32,33,34,35,36,37,38,39]. Hence initially getting precise estimates for upper marginal dimensionality n + (m = {2, 3}, 4 − ) is of physical importance to determine the type of phase transition in real systems.…”
Section: O(n) × O(m) Spin Modelsmentioning
confidence: 99%