Functionalized Polymeric Materials for Catalytic Upgrading of Biobased Feedstocks

Zhang, Heng; Xu, Chunbao; Yang, Song

doi:10.1155/2021/5036404

Cited by 1 publication

(1 citation statement)

References 8 publications

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“…Biomass, a kind of carbon-neutral energy source by absorbing CO 2 from the atmosphere through photosynthesis, is a vital renewable resource that is abundant on Earth and can be utilized to produce a diverse range of biomaterials and bioenergy, meeting the diverse development needs of modern society. 14,158,159 After processing, biomass raw materials could produce different biomass-derived molecules such as 5-hydroxymethylfurfural (HMF), 160 α-hydroxy acids, and α-keto acids. 161,162 These biomass-derived molecules could be further transformed into fine chemicals that are conventionally produced from fossil fuel resources.…”

Section: Electrocatalytic C─n Coupling Of Biomassmentioning

confidence: 99%

Toward effective electrocatalytic C–N coupling for the synthesis of organic nitrogenous compounds using CO₂ and biomass as carbon sources

Jiang,

Wu,

Zhang

et al. 2023

SusMat

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Thermochemical conversion of fossil resources into fuels, chemicals, and materials has rapidly increased atmospheric CO2 levels, hindering global efforts toward achieving carbon neutrality. With the increasing push for sustainability, utilizing electrochemical technology to transform CO2 or biomass into value‐added chemicals and to close the carbon cycle with sustainable energy sources represents a promising strategy. Expanding the scope of electrosynthesis technology is a prerequisite for the electrification of chemical manufacturing. To this end, constructing the C─N bond is considered a priority. However, a systematic review of electrocatalytic processes toward building C─N bonds using CO2 and biomass as carbon sources is not available. Accordingly, this review highlights the research progress in the electrosynthesis of organic nitrogen compounds from CO2 and biomass by C─N coupling reactions in view of catalytic materials, focusing on the enlightenment of traditional catalysis on C─N coupling and the understanding of the basis of electrochemical C─N coupling. The possibility of C─N bond in electrocatalysis is also examined from the standpoints of activation of substrates, coupling site, mechanism, and inhibition of hydrogen evolution reaction (HER). Finally, the challenges and prospects of electrocatalytic C─N coupling reactions with improved efficiency and selectivity for future development are discussed.

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Section: Electrocatalytic C─n Coupling Of Biomassmentioning

confidence: 99%

Toward effective electrocatalytic C–N coupling for the synthesis of organic nitrogenous compounds using CO₂ and biomass as carbon sources

Jiang,

Wu,

Zhang

et al. 2023

SusMat

Self Cite

View full text Add to dashboard Cite

show abstract

Functionalized Polymeric Materials for Catalytic Upgrading of Biobased Feedstocks

Cited by 1 publication

References 8 publications

Toward effective electrocatalytic C–N coupling for the synthesis of organic nitrogenous compounds using CO₂ and biomass as carbon sources

Toward effective electrocatalytic C–N coupling for the synthesis of organic nitrogenous compounds using CO₂ and biomass as carbon sources

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Functionalized Polymeric Materials for Catalytic Upgrading of Biobased Feedstocks

Cited by 1 publication

References 8 publications

Toward effective electrocatalytic C–N coupling for the synthesis of organic nitrogenous compounds using CO2 and biomass as carbon sources

Toward effective electrocatalytic C–N coupling for the synthesis of organic nitrogenous compounds using CO2 and biomass as carbon sources

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Product

Resources

About

Toward effective electrocatalytic C–N coupling for the synthesis of organic nitrogenous compounds using CO₂ and biomass as carbon sources

Toward effective electrocatalytic C–N coupling for the synthesis of organic nitrogenous compounds using CO₂ and biomass as carbon sources