This paper proposes the gain enhancement of dual-band and dual-polarized asymmetric horn antenna for the secondary radar system using hybrid metamaterial techniques. The hybrid metamaterial is comprised of the structures of woodpile electromagnetic bandgap (EBG) for gain enhancement of the primary main beam of the radar system at the operating frequency of 1,300 MHz with horizontal polarization; and the wire medium structure that is placed beside the EBG structure for gain improvement of the identification friend or foe (IFF) main beam, which is operated at the center frequency of 1,060 MHz with vertical polarization. Meanwhile, the cooperated structures have to function to control the directions of the primary and IFF main beams retaining at 0° and 6°, respectively, too. When the hybrid metamaterial structure is placed at the front of an asymmetric horn’s aperture, with suitable parameters and optimized spacing, it is found to increase the gains of the two beams compared to the single asymmetric horn around 3 dB and retain the directions of original main beams. The comparison of the results between simulation and measurement, such as the reflected power (S<sub>11</sub>), gain, and radiation patterns, are in good agreement.