We present the VLA-COSMOS 3 GHz Large Project based on 384 h of observations with the Karl G. Jansky Very Large Array (VLA) at 3 GHz (10 cm) toward the two square degree Cosmic Evolution Survey (COSMOS) field. The final mosaic reaches a median rms of 2.3 µJy beam −1 over the two square degrees at an angular resolution of 0.75 . To fully account for the spectral shape and resolution variations across the broad (2 GHz) band, we image all data with a multiscale, multifrequency synthesis algorithm. We present a catalog of 10 830 radio sources down to 5σ, out of which 67 are combined from multiple components. Comparing the positions of our 3 GHz sources with those from the Very Long Baseline Array (VLBA)-COSMOS survey, we estimate that the astrometry is accurate to 0.01 at the bright end (signal-to-noise ratio, S /N 3 GHz > 20). Survival analysis on our data combined with the VLA-COSMOS 1.4 GHz Joint Project catalog yields an expected median radio spectral index of α = −0.7. We compute completeness corrections via Monte Carlo simulations to derive the corrected 3 GHz source counts. Our counts are in agreement with previously derived 3 GHz counts based on single-pointing (0.087 square degrees) VLA data. In summary, the VLA-COSMOS 3 GHz Large Project simultaneously provides the largest and deepest radio continuum survey at high (0.75 ) angular resolution to date, bridging the gap between last-generation and next-generation surveys.