SummaryThe Department of Homeland Security and others rely on results from atmospheric dispersion models for threat evaluation, event management, and post-event analyses. The ability to simulate dry deposition rates is a crucial part of our emergency preparedness capabilities. Deposited materials pose potential hazards from radioactive shine, inhalation, and ingestion pathways. A reliable characterization of these potential exposures is critical for management and mitigation of these hazards.A review was conducted of the current status of dry deposition formulations used in these atmospheric dispersion models. The formulations for dry deposition of particulate materials considered an event such as a radiological attack involving a Radiological Detonation Device (RDD). The results of this effort are applicable to current emergency preparedness capabilities, such as are deployed in the Interagency Modeling and Atmospheric Assessment Center (IMAAC), other similar national/regional emergency response systems, and stand-alone emergency response models.The review concludes that dry deposition formulations need to consider the full range of particle sizes, including: 1) the accumulation mode range (0.1 to 1 micron in diameter) and its minimum deposition velocity, 2) smaller particles (less than 0.01 micron diameter) deposited mainly by molecular diffusion, 3) 10 to 50 micron diameter particles deposited mainly by impaction and gravitational settling, and 4) larger particles (greater than 100 micron diameter) deposited mainly by gravitational settling. The effects of the local turbulence intensity, particle characteristics, and surface element properties must also be addressed in the formulations.Specific improvements recommended for dry deposition formulations are 1) the capability of simulating near-field dry deposition patterns, 2) the capability of addressing the full range of potential particle properties, 3) the incorporation of particle surface retention/rebound processes, and 4) the development of dry deposition formulations applicable to urban areas. Also, to improve dry deposition modeling capabilities, atmospheric dispersion models in which the dry deposition formulations are imbedded need better source-term plume initialization and improved in-plume treatment of particle growth processes.Dry deposition formulations used in current models are largely inapplicable to the complex urban environment. An improved capability is urgently needed to provide surface-specific information to assess local-exposure hazard levels in both urban and non-urban areas on roads, buildings, crops, rivers, etc.A model improvement plan is developed with a near-term and far-term component. Despite some conceptual limitations, the current formulations for particle deposition based on a resistance approach have proven to be reasonable dry deposition simulations. For many models with inadequate dry deposition formulations, adding or improving a resistance approach will be the desirable near-term update. Resistance models, however, are i...