The 35S content in atmospheric deposition, aerosol and rain water was determined about every 10 days for a year with 7Be, 32p and some stable elements. Average 35S concentrations were l l0mBq-m-2-d -1 for atmospheric deposition, 0.078 mBq.m -3 for aerosol in surface air and 45 mBq-I -j for rain water. The ratios of 7Be/35S were abnormally low, although most of 32p/TBe showed the reasonable values corresponding to the residence times from 10 to 60 days. The excess 35S suggests an external source 0f35S or/and a faster cycle of 35S than that of TBe and 32p.