“…As a result, there is growing interest in taking inspiration directly from nature in order to develop sustainable and highly functional biobased materials. Due to their biocompatibility, biodegradability, and a range of chemical functionalities, these biobased materials have attracted significant attention in a wide range of fields such as biomedical, renewable energy, cultural heritage preservation, and building technology, representing a sustainable alternative to petroleum-based resources. − Cellulose and proteins are two of the most abundant biopolymers on Earth, playing diversified roles in many biological systems − and, as a result, are commonly used as natural building blocks in the preparation of biobased materials such as hydrogels and aerogels. In particular, due to their light weight, high specific surface area, and porous structure, aerogels commonly find application as oil/chemical absorbents, thermal insulators, biomedical scaffolds, and biocatalysts; however, before reaching practical application, the fundamental properties and interactions within biobased aerogels need to be thoroughly investigated…”