Given the complex spatiotemporal variability of aerosols, high-frequency satellite observations are essential for accurately mapping their distribution. However, optical remote sensing encounters difficulties in detecting Aerosol Optical Depth (AOD) over cloud-covered regions, creating data gaps that limit comprehensive environmental analysis. This study introduces a spatial gap-filling method for Himawari-8/Advanced Himawari Imager (AHI) hourly AOD data, using a Random Forest (RF) model that integrates meteorological variables and model-based AOD data. Developed and validated over South Korea from 1 January to 31 December 2019, the model effectively improved data coverage from 6% to 100%. The approach demonstrated high performance in blind tests, achieving a root mean square error (RMSE) of 0.064 and a correlation coefficient (CC) of 0.966. Meteorological analysis indicated optimal model performance under cold, dry conditions (RMSE: 0.047, CC: 0.956), compared to humid conditions (RMSE: 0.105, CC: 0.921). Validation against Aerosol Robotic Network (AERONET) ground observations showed that, while the original Himawari-8 data exhibited higher accuracy (RMSE: 0.189, CC: 0.815, n = 346), the gap-filled dataset maintained reasonable precision (RMSE: 0.208, CC: 0.711) and significantly increased the number of valid data points (n = 4149). Furthermore, the gap-filled dataset successfully captured seasonal AOD patterns, with values ranging from 0.245–0.300 in winter to 0.381–0.391 in summer, providing a comprehensive view of aerosol dynamics across South Korea.