Most Maquereau Group lavas are tholeiitic basalts that exhibit an Fe-Ti-enrichment trend. The tholeiites are divisible into incompatible-element-enriched and depleted types. Enriched tholeiites have chondrite-normalized La/Yb > 1 and higher incompatible element contents than do depleted, normal mid-ocean ridge basalt-like tholeiites. Subordinate transitional-alkaline basalts are even more enriched in TiO 2 , P 2 O 5 , Nb, and light rare-earth elements (REE). Intrasuite geochemical variations are consistent with coupled fractional crystallization and assimilation of Grenvillean continental crust or sediments derived therefrom. Assimilation leads to the development of characteristic enrichment in Ba, Th, Zr, and light REE. Intersuite variations cannot be accounted for through crystal fractionation or crustal contamination, and must reflect either source-mantle heterogeneity or mantle melting processes. Most major-and trace-element paleotectonic discriminants do not favor an arc-related environment for these lavas. An intracontinental rift or an incipient spreading ridge environment are most consistent with the geochemical data and field relationships.