Giant oligomeric porous cage-based molecules

Cortés-Martínez, Alba; von Baeckmann, Cornelia; Hernández-López, Laura; Carné-Sánchez, Arnau; Maspoch, Daniel

doi:10.1039/d4sc01974a

Chem. Sci.

2024

DOI: 10.1039/d4sc01974a

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Giant oligomeric porous cage-based molecules

Alba Cortés-Martínez,

Cornelia von Baeckmann,

Laura Hernández-López

et al.

Abstract: Most reported porous materials are either extended networks or monomeric discrete cavities; indeed, porous structures of intermediate size have scarcely been explored. Herein, we present the stepwise linkage of discrete...

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Metal‐Organic Cages: Synthetic Strategies and Photocatalytic Application

Liu,

Huang,

Qin

et al. 2024

ChemCatChem

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Metal‐organic cages (MOCs) are a class of compounds formed through the coordination of metal ions with organic ligands to create well‐defined and cage‐like structure. These unique structures offer versatile environments for catalyzing a wide range of chemical reactions. The catalytic capabilities of MOCs are significantly influenced by the nature of the metal ions, functional ligands, and the cage structure. Notably, the confined spaces within MOCs can lead to enhanced reaction efficiencies, particularly in processes such as light‐induced hydrogen generation and the photocatalytic reduction of CO2. Furthermore, MOCs show great potential in photo‐organic synthesis due to the cage structure which provide a confined environment, and allow for encapsulating organic molecules, making them useful for improving the selectivity and efficiency of catalytic process. This review reports the development of MOCs for photocatalysis, focusing on the structural design and regulation strategy to build functional MOCs for photocatalytic hydrogen production, CO2 reduction, organic transformation. Insights into the photocatalysis are discussed including the challenges and further research direction in MOC‐based photocatalysis.

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Metal‐Organic Cages: Synthetic Strategies and Photocatalytic Application

Liu,

Huang,

Qin

et al. 2024

ChemCatChem

View full text Add to dashboard Cite

show abstract

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Giant oligomeric porous cage-based molecules

Abstract: Most reported porous materials are either extended networks or monomeric discrete cavities; indeed, porous structures of intermediate size have scarcely been explored. Herein, we present the stepwise linkage of discrete...

Cited by 1 publication

References 48 publications

Metal‐Organic Cages: Synthetic Strategies and Photocatalytic Application

Metal‐Organic Cages: Synthetic Strategies and Photocatalytic Application

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