Radionuclide 239+240Pu dating and sedimentation
rate
is a crucial parameter for studying lake sedimentary processes. To
comprehensively investigate 239+240Pu vertical distributions
and relevant processes in Chinese lakes, this study collects and summarizes
54 sediment core samples from 40 lakes and reservoirs globally. First,
the results suggest that two typical vertical distributions of 239+240Pu are summarized in Chinese lakes. The location of
the 239+240Pu peak corresponds to the age of global atmospheric
nuclear test deposition in 1963 ± 1. Second, 239+240Pu based on 1963 peak is far more suitable for lake dating compared
to 137Cs, and a significant linear correlation (R
2 = 0.924) between the depth of 239+240Pu maximum value (cm) and sedimentation rate (cm a–1) in Chinese lakes was established. For the first time, this study
has found that this significant linear relationship can be generalized
globally (R
2 = 0.909), regardless of where
the lake sediment cores were sampled. Third, we identify three typical
vertical distributions for the 240Pu/239Pu atom
ratio in Chinese lake sediment cores: invariant distribution, mutation
distribution, and gradient distribution. This result implies that 239+240Pu in Chinese lakes mainly originate from the global
fallout; yet this does not rule out the potential contribution from
local sources of 239+240Pu, such as the Lop Nor nuclear
tests, the atomic city nuclear activities, and the Chernobyl nuclear
accident. However, the trend in the average 240Pu/239Pu ratio varies independent of latitude. Moreover, a significant
positive linear correlation is detected between average 239+240Pu inventory in the soil and lake cores, with a coefficient of 0.538.
In particular, the high 239+240Pu inventory background
value in Northwest China closely correlates with the deposition of 239+240Pu in some lakes (e.g., Lake Sugan). This manuscript
provides insights into 239+240Pu vertical patterns and
processes in Chinese lakes and sheds light on future research using 239+240Pu for dating and sedimentation rate in lakes outside
China.