2024
DOI: 10.1021/acsapm.4c01454
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Glycidyl Ether-Functionalized Poly(ethylenimine)-Impregnated Sorbents for CO2 Capture from Ultradilute Sources

Samser Shaikh,
Stephanie A. Didas,
Miles A. Sakwa-Novak
et al.

Abstract: Carbon dioxide adsorbents based on branched poly(ethylenimine) (PEI) are prevalent in postcombustion CO 2 capture as well as direct air capture (DAC) of CO 2 . In DAC, PEI-based sorbents offer good tolerance to ranging environmental conditions (temperature, relative humidity, etc.) but require moderate temperature swings for CO 2 desorption and oxidize over extended cycling in oxidative environments, such as ambient air. In this work, the functionalization of branched PEI with epoxides and glycidyl ethers of v… Show more

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