“…This differs from our previous estimate of two Au chains per unit cell and greatly narrows the range of other published coverage estimates of 2-4 chains per unit cell. 12,27,28,33,35,[37][38][39][40][41][42][43][44][45] A similar analysis for the Si͑553͒-Au surface yields a coverage of 2.1Ϯ 0.4 chains per unit cell, which is again higher than previously estimated but consistent with the coverage of two Au chains per unit cell obtained from x-ray diffraction. 46 In light of this coverage determination, most of the published structural models for Si͑553͒-Au and Si͑111͒ 5 ϫ 2-Au will require revision to accommodate an additional gold chain.…”