NiZn ferrite nanoparticles (2−20 wt %) of composition Ni 0.4 Zn 0.6 Fe 2 O 4 were introduced into LiZnTi ferrite of composition Li 0.42 Zn 0.27 Ti 0.11 Fe 2.2 O 4 and sintered at a temperature of 920°C for 2 h, well below that of the Ag melting point. Here, LiZnTi ferrites were prepared by a solidstate reaction method, and NiZn ferrite nanoparticles were fabricated by a hydrothermal chemical technique at 180°C. A low ferromagnetic resonance (FMR) line width, low coercivity, and high magnetic moment were achieved after refinement of the heat treatment conditions of the mixture. Riveted full profile refinement of the X-ray powder diffraction patterns and analysis of Mossbauer spectra were employed to study the structure and caption distribution. The results confirm a pure spinel phase after processing. A narrow FMR line width of 152.5 Oe, a reduced coercivity of 132.9 A/m, and an improved saturation magnetization of 74.23 emu/g were obtained by way of the addition of 8 wt % NiZn ferrite nanoparticles.