Graphene environmental footprint greatly reduced when derived from biomass waste via flash Joule heating

Jia, Chao; Pang, Mingyue; Lu, Yuanda; Liu, Yize; Zhuang, Minghao; Liu, Beibei; Wei, Tao; Wang, Liang; Bian, Ting; Wang, Meiling; Yu, Fengbo; Sun, Liming; Lin, Litao; Teng, Tao; Wu, Xuan; He, Zhelin; Gao, Jie; Luo, Jun; Zhang, Shicheng; Feng, Lei; Yin, Xinhan; You, Fengqi; Li, Gang; Zhang, Lixiao; Zhu, Yun; Zhu, Xiangdong; Yi, Yang

doi:10.1016/j.oneear.2022.11.006

Cited by 33 publications

(21 citation statements)

References 55 publications

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“…The test methods of the voltage, current, and temperature profile in the FJH process have been reported in our previous work. 24 Other characterizations used to simulate the temperature distribution in the FJH process were also detailed in Text S4 and Table S2.…”

Section: ■ Materials and Methodsmentioning

confidence: 99%

Joule Heating Induced Reductive Iron–Magnesium Bimetallic Nanocomposite for Eminent Heavy Metal Removal

Jia,

Sun,

et al. 2024

ACS EST Eng.

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Fe 0 -based materials exhibit great power in removing heavy metals, but their passivation issues remain a challenge. Guided by the synergistic effects within bimetallic modifications, a novel reductive FeMg bimetallic nanocomposite (FeMg/NC) was constructed using flash Joule heating technology. The ultrafast heating and quenching process achieved a phase-fusional structure comprising Fe 0 and Mg 0 encapsulated in the resulting aromaticcarbon layer. Incorporation of highly reductive Mg 0 into Fe 0 -based material led to an approximately 2−3 times enhancement in pollutant removal efficiency compared to monometallic nanocomposites. Experiments and theoretical calculations revealed that this augmented removal efficiency arose from the FeMg dual-site synergistic effect, facilitating the interaction between FeMg/NC and the targeted pollutants. That is, adsorption led to the directional inward diffusion of pollutants, and the outward release of electrons from this formed phase-fusion structure was accelerated via the electron delocalization effect. Therefore, FeMg/NC exhibited excellent removal capacities for typical heavy metals (including Cr(VI), Sb(V), Ni(II), and Cu(II)). This study demonstrates the flexibility of Joule heating technology for constructing bimetallic nanocomposite, which can effectively address heavy metal pollution and opens up endless possibilities for developing more impactful environmental remediation materials.

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Section: ■ Materials and Methodsmentioning

confidence: 99%

Joule Heating Induced Reductive Iron–Magnesium Bimetallic Nanocomposite for Eminent Heavy Metal Removal

Jia,

Sun,

et al. 2024

ACS EST Eng.

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“…Additionally, the energy-intensive nature of the production process contributes to greenhouse gas emissions and resource depletion. [233][234][235][236] To address these concerns, researchers are actively exploring greener synthesis routes for GO production. 44,237 For instance, some studies have investigated the use of environmentally friendly solvents and mild oxidizing agents to minimize the ecological footprint of the process.…”

Section: Environmental Impacts and Sustainability Of Go In Sc Technologymentioning

confidence: 99%

Recent advances in energy storage with graphene oxide for supercapacitor technology

Mousavi,

Hashemi,

Kalashgrani

et al. 2023

Sustainable Energy Fuels

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“…3). In addition, there also has been research that reported the use of laser, 55 microwave-assisted, 56 plasma, 57 and flash Joule heating 58 to obtain biochar from biomass. Several reactions are contained during the carbonization of biomass normally, including dehydration, decarboxylation, depolymerization, isomerization, and aromatization.…”

Section: Carbonization Of Biomassmentioning

confidence: 99%

Biomass-derived 2D carbon materials: structure, fabrication, and application in electrochemical sensors

Xiao,

Li,

Deng

et al. 2023

J. Mater. Chem. B

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Graphene environmental footprint greatly reduced when derived from biomass waste via flash Joule heating

Cited by 33 publications

References 55 publications

Joule Heating Induced Reductive Iron–Magnesium Bimetallic Nanocomposite for Eminent Heavy Metal Removal

Joule Heating Induced Reductive Iron–Magnesium Bimetallic Nanocomposite for Eminent Heavy Metal Removal

Recent advances in energy storage with graphene oxide for supercapacitor technology

Biomass-derived 2D carbon materials: structure, fabrication, and application in electrochemical sensors

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