Green and eco-friendly porous imprinted hydrogels with cellulose nanocrystals-based precise-designed hyperbranched sites for high-accuracy separation and purification of naringin

Liu, Shucheng; Tang, Nana; Huang, Hao; Zhang, Xuan; Lu, Ruiheng; Li, Yuheng

doi:10.1016/j.cej.2024.152821

Chemical Engineering Journal

2024

DOI: 10.1016/j.cej.2024.152821

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Green and eco-friendly porous imprinted hydrogels with cellulose nanocrystals-based precise-designed hyperbranched sites for high-accuracy separation and purification of naringin

Shucheng Liu,

Nana Tang,

Hao Huang

et al.

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Cited by 5 publications

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Steerable Interfacial Assembly of 1D Amyloid‐Like Protein Nanocomposites for Enhanced Nanoherbicide Utilization

Yu,

Chen,

Zhang

et al. 2024

Small

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Conventional herbicide formulations suffer from serious problems such as easy drift, run‐off and scouring into the environment, which pose enormous threats to human health and environmental safety. Herein, an innovative strategy is proposed to prepare oil‐in‐water nanoemulsions with long‐term stability, enhanced droplet deposition, and improved nanoherbicide adhesion via steerable interfacial assembly of 1D amyloid‐like protein nanocomposites. Bovine serum albumin (BSA) undergoes rapid amyloid‐like aggregation upon reduction of its disulfide bond. The resulting phase‐transitioned BSA (PTB) oligomers instantly self‐assemble on the surface of cellulose nanofibers (CNF) to form the 1D PTB/CNF nanocomposites, which greatly expands the parameter space for interfacial assembly of amyloid‐like proteins. The PTB/CNF nanocomposites exhibit excellent interfacial activity, enabling spontaneous adsorption at the oil‐water interface to stabilize nanoemulsion. The excess PTB/CNF nanocomposites would also self‐assemble at the air‐aqueous interface upon spraying, resulting in efficient droplet deposition on (super)hydrophobic leaves. The deposited nanoherbicides show excellent resistance to wind/rain corrosion due to the robust amyloid‐mediated adhesion, with a retention rate of more than 80% after severe scouring. Consequently, herbicide applications can be reduced by at least 30% compared to commercial emulsifiable concentrates, showing greater herbicidal efficiency. This study provides novel insights and approaches to promote sustainable agricultural development.

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Steerable Interfacial Assembly of 1D Amyloid‐Like Protein Nanocomposites for Enhanced Nanoherbicide Utilization

Yu,

Chen,

Zhang

et al. 2024

Small

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Nanoscale engineer: The revolutionary role of nanobubbles in the synthesis of functional nanomaterials

Wu,

Zhang,

et al. 2025

Desalination

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Efficient adsorption of flavonoids on amino-functionalized ZIF-8/chitosan aerogels

Zhang,

Ma,

et al. 2024

International Journal of Biological Macromolecules

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Green and eco-friendly porous imprinted hydrogels with cellulose nanocrystals-based precise-designed hyperbranched sites for high-accuracy separation and purification of naringin

Cited by 5 publications

References 56 publications

Steerable Interfacial Assembly of 1D Amyloid‐Like Protein Nanocomposites for Enhanced Nanoherbicide Utilization

Steerable Interfacial Assembly of 1D Amyloid‐Like Protein Nanocomposites for Enhanced Nanoherbicide Utilization

Nanoscale engineer: The revolutionary role of nanobubbles in the synthesis of functional nanomaterials

Efficient adsorption of flavonoids on amino-functionalized ZIF-8/chitosan aerogels

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