2017
DOI: 10.1063/1.4978755
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Heterodyne technique in photoinduced force microscopy with photothermal effect

Abstract: The heterodyne technique is used to detect short-range forces. Using the heterodyne technique, we demonstrate photoinduced force microscopy (PiFM) imaging and z-spectroscopy without the artifact of photothermal vibration. The rejection ratio was at least 99.975% under a high-scattering condition. In addition, the heterodyne technique employs the optimal amplitude at the first resonance frequency of the cantilever to detect the photoinduced force sensitively. According to our calculation, the optimal ratio of t… Show more

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Cited by 29 publications
(29 citation statements)
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“…The first eigenmode of the cantilever is excited by the interaction forces between the sample and the tip, which are induced by the external laser source. This interaction is detected in the cantilever mechanics when the laser intensity is modulated at the frequency difference between the first and second eigenmode resonances 20 , 21 . In this case, the laser (QCL from Block Engineering) is p-polarized, the pulse width is 20 ns, and the light wavenumber (wavelength) can be tuned between 795 and 1900 cm −1 .…”
Section: Resultsmentioning
confidence: 98%
“…The first eigenmode of the cantilever is excited by the interaction forces between the sample and the tip, which are induced by the external laser source. This interaction is detected in the cantilever mechanics when the laser intensity is modulated at the frequency difference between the first and second eigenmode resonances 20 , 21 . In this case, the laser (QCL from Block Engineering) is p-polarized, the pulse width is 20 ns, and the light wavenumber (wavelength) can be tuned between 795 and 1900 cm −1 .…”
Section: Resultsmentioning
confidence: 98%
“…The numerical analyses reveal that due to their phase difference, photothermal and photovoltage effects add or subtract their action on the cantilever, depending on the DC field sign. These findings are of relevance for all AFM techniques which use an optical excitation of the cantilever sensor, and for the emergent field of photoinduced force microscopy [31][32][33][34][35] in particular, as well as for other opto-mechanical systems where intrinsic or externally controlled electrostatic fields and light absorption are involved.…”
mentioning
confidence: 75%
“…213, 214 This heterodyne detection is reported to improve imaging contrast, as compared to direct detection at the modulation frequency (f m ), and effectively avoid artifacts caused by photothermal effects. 215 Figure 10 shows a general schematic of PiFM experimental setup. More theoretical details and early experiments of PiFM are summarized in previous reports.…”
Section: Pifmmentioning
confidence: 99%