Triboelectric
nanogenerators (TENGs) are newly developed energy-harvesting
mechanisms, which can efficiently transmute irregular mechanical energy
into scarce electrical energy. However, the electrical performance
of TENGs shows a decreasing tendency with the increase in temperature,
and the negative effect caused by friction heat and operating environmental
thermal stresses for the output performance, durability, and reliability
are still a bottleneck, restricting the practical application of TENG
electronic devices. Especially for wearable TENG devices, the heat-induced
temperature rise evokes extreme discomfort and even hazards to human
health. To effectively suppress the thermal negative effect and maintain
the high-temperature steady electrical performance of TENGs, a novel
thermo-regulating TENG (Tr-TENG) based on phase change materials (PCMs)
is designed. The results state clearly that the Tr-TENG can maintain
steady output performance without deterioration by the introduction
of PCMs, during continuous heating and natural cooling, while the
output performance of conventional TENG is decayed by 18.33%. More
importantly, the Tr-TENG possesses high-efficiency thermal management
ability, resulting in its improved durability, reliability, and thermal
comfort. This study creates new possibilities for the development
of advanced multifunctional TENGs with attractive characteristics
and desirable performances and promotes the application of TENG electronic
devices in harsh environments.