High-entropy perovskite oxide washcoated porous alumina ceramic as a superb catalyst for activating peroxymonosulfate to eliminate refractory organic pollutants

Han, Bo; Pan, Qihui; Chen, Yuhao; Liu, Ding; Zhou, Chenggang; Xia, Kaisheng; Gao, Qiang

doi:10.1016/j.cej.2022.140828

Chemical Engineering Journal

2023

DOI: 10.1016/j.cej.2022.140828

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High-entropy perovskite oxide washcoated porous alumina ceramic as a superb catalyst for activating peroxymonosulfate to eliminate refractory organic pollutants

Bo Han

Qihui Pan

Yuhao Chen

et al.

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Cited by 16 publications

References 68 publications

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Nanoporous High Entropy Alloy Al‐Pt‐Pd‐Ru as an Efficient Catalyst for One‐Pot Reductive Amination of Nitroarenes

Wang,

et al. 2024

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High entropy alloys (HEAs) are promising heterocatalysts because of their unique physicochemical properties, but research on HEA‐catalyzed tandem reactions is lacking. Moreover, limited research on HEAs for molecular transformation has hindered their development. Herein, an unsupported nanoporous HEA Al‐Pt‐Pd‐Ru (HEANPore) prepared using a top‐down dealloying method is reported. The Lewis acidity and electron redistribution of the noble metals Pt, Pd, and Ru are identified to be intrinsic of high activity and selectivity of HEANPore in the one‐pot reductive amination of nitroarenes. The competitive adsorption of the reactant and corresponding reaction mechanism are investigated using DFT. This study demonstrates the exceptional performance of the HEANPore in tandem reactions, presenting new possibilities for the application of HEAs in the field of catalysis.

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Nanoporous High Entropy Alloy Al‐Pt‐Pd‐Ru as an Efficient Catalyst for One‐Pot Reductive Amination of Nitroarenes

Wang,

et al. 2024

Small

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High-entropy alloy nanoparticles/biochar as an efficient catalyst for high-performance treatment of organic pollutants

Miao

Guo

Liu

et al. 2023

Chemical Engineering Journal

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Combination of co-doped Ce-Mn perovskite with different spacial distributions for methane catalytic reforming reactor to realize functional partition

Dai,

Wang

2023

Chemical Engineering Journal

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High-entropy perovskite oxide washcoated porous alumina ceramic as a superb catalyst for activating peroxymonosulfate to eliminate refractory organic pollutants

Cited by 16 publications

References 68 publications

Nanoporous High Entropy Alloy Al‐Pt‐Pd‐Ru as an Efficient Catalyst for One‐Pot Reductive Amination of Nitroarenes

Nanoporous High Entropy Alloy Al‐Pt‐Pd‐Ru as an Efficient Catalyst for One‐Pot Reductive Amination of Nitroarenes

High-entropy alloy nanoparticles/biochar as an efficient catalyst for high-performance treatment of organic pollutants

Combination of co-doped Ce-Mn perovskite with different spacial distributions for methane catalytic reforming reactor to realize functional partition

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