“…After we have excluded non‐uniformities in magnetic moment density, electron scattering strength, and exchange stiffness as the dominant mechanisms of inversion asymmetry, the lattice strain gradient is left as the most likely symmetry‐breaking mechanism for the bulk dampinglike SOT. Microscopically, a strain gradient can non‐uniformly modify the strengths of the SHE, [ 31–35 ] spin‐orbit interaction, [ 36 ] orbital polarization, [ 37 ] spin states at the Fermi level, [ 37 ] and strain‐spin coupling, [ 38 ] ultimately leading to inversion symmetry breaking in the generation and relaxation of spin current within the sample. As shown in Figure 4c, the lattice constant of the chemically disordered Fe x Pt 1‐ x indeed increases by 2.3% as x from 0.25 to 0.75, [ 39 ] suggesting a very strong strain gradient in the composition‐gradient samples.…”