“…In the last decade, there has been a growing interest to extend high harmonic generation (HHG) to twodimensional (2D) crystals and nanostructures, such as semimetallic graphene [1], and semiconductor transition metal dichalcogenidescite [2]. The role of graphene as an effective nonlinear optical material has been discussed in many theoretical [3][4][5][6][7][8][9][10][11][12][13][14][15][16][17][18][19][20], and experimental [23], [24] studies that consider various extreme nonlinear optical effects, in particular, HHG, which takes place in strong coherent radiation fields in the multiphoton regime at excitation of such nanostructures [25], [26]. On the other hand, apart from the remarkable and unique electronic and optical properties of graphene, the lack of an energy gap as a semimetal greatly limits their applicability, in contrast, for example, to bilayer graphene [27][28][29][30][31][32].…”