Next-generation mobile communication systems are planned to support millimeter Wave (mmWave) transmission in scenarios with high-mobility, such as in private industrial networks. To cope with propagation environments with unprecedented challenges, data-driven methodologies such as Machine Learning (ML) are expected to act as a fundamental tool for decision support in future mobile systems. However, highquality measurement datasets need to be made available to the research community in order to develop and benchmark MLbased methodologies for next-generation wireless networks. We present a reliable testbed for collecting channel measurements at sub-6 GHz and mmWave frequencies. Further, we describe a rich dataset collected using the presented testbed. Our public dataset enables the development and testing of innovative ML-based channel simulators for both sub-6 GHz and mmWave bands on real-world data. We conclude this paper by discussing promising experimental results on two illustrative ML tasks leveraging on our dataset, namely, channel impulse response forecasting and synthetic channel transfer function generation, upon which we propose future exploratory research directions. The original dataset employed in this work is available on IEEE DataPort 1 , and the code utilized in our numerical experiments is publicly accessible via CodeOcean 2 Index Terms-machine learning, deep learning, radio channel prediction, radio channel simulation, vehicular communications, channel sounding, channel measurements.