“…Since only few MIR broadband laser gain media exist [11,15,24], many sources rely on nonlinear frequency conversion [18,25]. Among numerous frequency conversion methods utilizing χ (2) and χ (3) nonlinearities in materials, difference frequency generation (DFG) is a widely used method [4,7,14,17,20,23]. In the DFG method two near infrared (NIR) laser pulses, the pump and signal pulse interact in a χ (2) nonlinear crystal material and generate a MIR idler pulse, conserving photon energy and momentum [1].…”