High strength, self-healing and hydrophobic fully bio-based polybenzoxazine reinforced pine oleoresin-based vitrimer and its application in carbon fiber reinforced polymers

Zhou, Xuan; Shen, Minggui; Fu, Fei; Li, Qiaoguang; Liu, He; Song, Zhanqian

doi:10.1016/j.cej.2024.149585

Chemical Engineering Journal

2024

DOI: 10.1016/j.cej.2024.149585

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High strength, self-healing and hydrophobic fully bio-based polybenzoxazine reinforced pine oleoresin-based vitrimer and its application in carbon fiber reinforced polymers

Xuan Zhou,

Minggui Shen,

Fei Fu

et al.

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Cited by 7 publications

References 75 publications

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Bio‐Based Thermosetting Resins: From Molecular Engineering to Intrinsically Multifunctional Customization

Zhao,

Liu,

Wang

et al. 2024

Advanced Materials

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Recent years have witnessed a growing interest in bio‐based thermosetting resins in terms of environmental concerns and the desire for sustainable industrial practices. Beyond sustainability, utilizing the structural diversity of renewable feedstock to craft bio‐based thermosets with customized functionalities is very worthy of expectation. There exist many bio‐based compounds with inherently unique chemical structures and functions, some of which are even difficult to synthesize artificially. Over the past decade, great efforts are devoted to discovering/designing functional properties of bio‐based thermosets, and notable progress have been made in antibacterial, antifouling, flame retardancy, serving as carbon precursors, and stimuli responsiveness, among others, largely expanding their application potential and future prospects. In this review, recent advances in the field of functional bio‐based thermosets are presented, with a particular focus on molecular structures and design strategies for discovering functional properties. Examples are highlighted wherein functionalities are facilitated by the inherent structures of bio‐based feedstock. Perspectives on issues regarding further advances in this field are proposed at the end.This article is protected by copyright. All rights reserved

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Bio‐Based Thermosetting Resins: From Molecular Engineering to Intrinsically Multifunctional Customization

Zhao,

Liu,

Wang

et al. 2024

Advanced Materials

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Dynamic Covalent Bonds Enabled Carbon Fiber Reinforced Polymers Recyclability and Material Circularity

Fan,

Zheng,

Yeo

et al. 2024

Angewandte Chemie

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Due to their remarkable features of lightweight, high strength, stiffness, high‐temperature resistance, and corrosion resistance, carbon fiber reinforced polymers (CFRPs) are extensively used in sports equipment, vehicles, aircraft, windmill blades, and other sectors. The urging need to develop a resource‐saving and environmentally responsible society requires the recycling of CFRPs. Traditional CFRPs, on the other hand, are difficult to recycle due to the permanent covalent crosslinking of polymer matrices. The combination of covalent adaptable networks (CANs) with carbon fibers (CFs) marks a new development path for closed‐loop recyclable CFRPs and polymer resins. This review summarizes the most recent developments of closed‐loop recyclable CFRPs from the unique paradigm of dynamic crosslinking polymers, CANs. These sophisticated materials with diverse functions, oriented towards CFs recycling and resin sustainability, are further categorized into several active domains of dynamic covalent bonds, including ester bonds, imine bonds, disulfide bonds, boronic ester bonds, and acetal linkages, etc. Finally, the possible strategies for the future design of recyclable CFPRs by combining dynamic covalent chemistry innovation with materials interface science are proposed.

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Dynamic Covalent Bonds Enabled Carbon Fiber Reinforced Polymers Recyclability and Material Circularity

Fan,

Zheng,

Yeo

et al. 2024

Angew Chem Int Ed

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High strength, self-healing and hydrophobic fully bio-based polybenzoxazine reinforced pine oleoresin-based vitrimer and its application in carbon fiber reinforced polymers

Cited by 7 publications

References 75 publications

Bio‐Based Thermosetting Resins: From Molecular Engineering to Intrinsically Multifunctional Customization

Bio‐Based Thermosetting Resins: From Molecular Engineering to Intrinsically Multifunctional Customization

Dynamic Covalent Bonds Enabled Carbon Fiber Reinforced Polymers Recyclability and Material Circularity

Dynamic Covalent Bonds Enabled Carbon Fiber Reinforced Polymers Recyclability and Material Circularity

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